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Piezoelectric ink jet printing of horseradish peroxidase on fibrous substrates

2007· article· en· W4378446664 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueTechnical programs and proceedings/Technical program and proceedings · 2007
Typearticle
Languageen
FieldEngineering
Topic3D Printing in Biomedical Research
Canadian institutionsUniversity of Toronto
FundersNatural Sciences and Engineering Research Council of CanadaUniversity of Toronto
KeywordsHorseradish peroxidaseBioanalysisSubstrate (aquarium)Materials scienceABTSInkwellNanotechnologyChemical engineeringChemistryComposite materialOrganic chemistryEnzymeDPPH

Abstract

fetched live from OpenAlex

Solid phase bioanalysis relies on the creation of a highly selective and sensitive layer of bioagent on a solid support capable of recognizing specific target analytes. Using ink jet printing technology picoliter volumes of bioagents can be precisely patterned over large surfaces with controlled uniformity. Despite the advantages of bioanalytical methods and the flexibility of ink jet printers, producing this type of functional materials is challenging. Solid supports can affect the biological activity, the spatial distribution and the binding capacity of the bioagent causing problems during post print detection. In this study a bioink containing the enzyme horseradish peroxidase (HRP) was jetted with a piezoelectric-based ink-jet deposition system on various fibrous substrates with differences in composition, surface chemistry and pore structure. Enzyme activity in solution and after printing was tested colorimetrically using 2, 2′-azino-di-(3- ethylbenzthiazoline) 6-sulphonate (ABTS) as chromogen. It was found that the papers tested have significantly different bioanalytical response in the detection of hydrogen peroxide. The uncoated papers showed the most sensitive green color response; whereas, the uncoated wood free paper gave the broader range of measurement and the highest color intensity. In contrast, the coated papers developed lower color intensity and the cast coated paper produced a pink color response possibly due to enzyme intermediate compounds produced under conditions of substrate inhibition.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.003
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Other design · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.889
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0030.001
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.002
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0010.002
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.016
GPT teacher head0.274
Teacher spread0.258 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it