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Record W4378471948 · doi:10.3847/psj/acd32f

Depletion of <sup>13</sup>C in CO in the Atmosphere of Mars Suggested by ExoMars-TGO/NOMAD Observations

2023· article· en· W4378471948 on OpenAlexfundno aff
Shohei Aoki, Kimie Shiobara, Nao Yoshida, Loïc Trompet, Naoki Terada, Hiromu Nakagawa, Giuliano Liuzzi, Ann Carine Vandaele, Ian Thomas, Gerónimo Villanueva, M. Á. López‐Valverde, Adrián Brines, Manish Patel, Sara Faggi, Frank Daerden, Justin Erwin, Bojan Ristic, G. Bellucci, J. J. López‐Moreno, Hiroyuki Kurokawa, Yuichiro Ueno

Bibliographic record

VenueThe Planetary Science Journal · 2023
Typearticle
Languageen
FieldEnvironmental Science
TopicAtmospheric and Environmental Gas Dynamics
Canadian institutionsnot available
FundersInstituto de Astrofísica de AndalucíaMinisterio de Ciencia e InnovaciónAgenzia Spaziale ItalianaBelgian Federal Science Policy OfficeEuropean CommissionCanadian Space AgencyUK Space AgencyFonds De La Recherche Scientifique - FNRSJapan Society for the Promotion of ScienceMinisterio de Ciencia, Innovación y UniversidadesNational Aeronautics and Space Administration
KeywordsIsotopologueMars Exploration ProgramAtmosphere of MarsAtmosphere (unit)Analytical Chemistry (journal)Carbon monoxideCarbon dioxideSpectral lineOccultationStandard deviationMixing ratioTrace gasPhysicsAstrophysicsAtmospheric sciencesChemistryAstrobiologyMartianMeteorologyAstronomy

Abstract

fetched live from OpenAlex

Abstract The atmosphere of Mars is mainly composed by carbon dioxide (CO2). It has been predicted that photodissociation of CO2 depletes 13C in carbon monoxide (CO). We present the carbon 13C/12C isotopic ratio in CO at 30–50 km altitude from the analysis of the solar occultation measurements taken by the instrument Nadir and Occultation for Mars Discovery on board the ExoMars Trace Gas Orbiter (ExoMars-TGO). We retrieve 12C16O, 13C16O, and 12C18O volume mixing ratios from the spectra taken at 4112–4213 cm−1, where multiple CO isotope lines with similar intensities are available. The intensities of the 12C16O lines in this spectral range are particularly sensitive to temperature, thus we derive the atmospheric temperature by retrieving CO2 density with simultaneously measured spectra at 2966–2990 cm−1. The mean δ 13C value obtained from the 13C16O/12C16O ratios is −263‰, and the standard deviation and standard error of the mean are 132‰ and 4‰, respectively. The relatively large standard deviation is due to the strong temperature dependences in the 12C16O lines. We also examine the 13C16O/12C18O ratio, whose lines are less sensitive to temperature. The mean δ value obtained with 12C18O instead of 12C16O is −82‰ with smaller standard deviation, 60‰. These results suggest that CO is depleted in 13C when compared to CO2 in the Martian atmosphere as measured by the Curiosity rover. This depletion of 13C in CO is consistent with the CO2 photolysis-induced fractionation, which might support a CO-based photochemical origin of organics in Martian sediments.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.003
Threshold uncertainty score0.007

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.001
Science and technology studies0.0000.000
Scholarly communication0.0010.000
Open science0.0000.000
Research integrity0.0010.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.014
GPT teacher head0.213
Teacher spread0.200 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations9
Published2023
Admission routes1
Has abstractyes

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