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Record W4379015535 · doi:10.1002/cjce.24975

<scp>CO<sub>2</sub></scp> utilization for methanol production; Optimal pathways with minimum <scp>GHG</scp> reduction cost

2023· article· en· W4379015535 on OpenAlexaffvenue
Yaser Khojasteh Salkuyeh, Omid Ashrafi, Ehsan Mostafavi, Philippe Navarri

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2023
Typearticle
Languageen
FieldChemical Engineering
TopicCatalysts for Methane Reforming
Canadian institutionsNatural Resources CanadaConcordia University
Fundersnot available
KeywordsGreenhouse gasProduction (economics)MethanolTonneRaw materialLife-cycle assessmentEnvironmental scienceBusinessWaste managementPulp and paper industryChemistryEconomicsEngineeringMicroeconomics

Abstract

fetched live from OpenAlex

Abstract Mitigating CO 2 emissions from industries and other sectors of our economy is a critical component of building a sustainable economy. This paper investigates two different methanol synthesis routes based on CO 2 utilization (CO 2 capture and utilization [CCU], and tri‐reforming of methane [TRM]), and compares the results with the conventional methanol production using natural gas as the feedstock (NG‐MeOH). A comprehensive techno‐economic analysis (TEA) model that includes the findings of the life cycle assessment (LCA) models of methanol production using various CO 2 utilization pathways is conducted. Economic analysis is conducted by developing a cost model that is connected to the simulation models for each production route. Compared to the conventional process (with a GHG emission of 0.6 kg CO 2 /kg MeOH), the lifecycle GHG reduction of 1.75 and 0.41 kg CO 2 /kg MeOH are achievable in the CCU and TRM pathways, respectively. Furthermore, the results indicate that, under current market conditions and hydrogen production costs, methanol production via CO 2 hydrogenation will result in a cost approximately three times higher than that of the conventional process. The integrated TEA–LCA model shows that this increased cost of production equates to a required life cycle GHG reduction credit of $279 to $422 per tonne of CO 2 utilized, depending on construction material and selected pathway. Additionally, when compared to the CO 2 hydrogenation route, the tri‐reforming process (TRM‐MeOH) can result in a 42% cost savings. Furthermore, a minimum financial support of $56 per tonne utilized CO 2 will be required to make the TRM‐MeOH process economically viable.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.003
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.068
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.003
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.026
GPT teacher head0.228
Teacher spread0.203 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations14
Published2023
Admission routes2
Has abstractyes

Explore more

Same venueThe Canadian Journal of Chemical EngineeringSame topicCatalysts for Methane ReformingFrench-language works237,207