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Record W4380686780 · doi:10.1088/1367-2630/acd411

Efficient pathway to NaCs ground state molecules

2023· article· en· W4380686780 on OpenAlexfundno aff
Claire Warner, Niccolò Bigagli, Aden Z. Lam, Weijun Yuan, Siwei Zhang, Ian Stevenson, Sebastian Will

Bibliographic record

VenueNew Journal of Physics · 2023
Typearticle
Languageen
FieldPhysics and Astronomy
TopicCold Atom Physics and Bose-Einstein Condensates
Canadian institutionsnot available
FundersOffice of Naval Research GlobalNatural Sciences and Engineering Research Council of CanadaDivision of PhysicsColumbia UniversityCroucher FoundationAlfred P. Sloan Foundation
KeywordsPhysicsStimulated Raman adiabatic passageRotational–vibrational spectroscopyAtomic physicsMoleculeGround stateExcited stateAdiabatic processSpin (aerodynamics)Realization (probability)Molecular physicsQuantum mechanics

Abstract

fetched live from OpenAlex

Abstract We present a study of two-photon pathways for the transfer of NaCs molecules to their rovibrational ground state. Starting from NaCs Feshbach molecules, we perform bound-bound excited state spectroscopy in the wavelength range from 900 nm to 940 nm, covering more than 30 vibrational states of the <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" overflow="scroll"> <mml:msup> <mml:mi>c</mml:mi> <mml:mn>3</mml:mn> </mml:msup> <mml:msup> <mml:mi mathvariant="normal">Σ</mml:mi> <mml:mo>+</mml:mo> </mml:msup> </mml:math> , <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" overflow="scroll"> <mml:msup> <mml:mi>b</mml:mi> <mml:mn>3</mml:mn> </mml:msup> <mml:mi mathvariant="normal">Π</mml:mi> </mml:math> , and <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" overflow="scroll"> <mml:msup> <mml:mi>B</mml:mi> <mml:mn>1</mml:mn> </mml:msup> <mml:mi mathvariant="normal">Π</mml:mi> </mml:math> electronic states. Analyzing the rotational substructure, we identify the highly mixed <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" overflow="scroll"> <mml:msup> <mml:mi>c</mml:mi> <mml:mn>3</mml:mn> </mml:msup> <mml:msubsup> <mml:mi mathvariant="normal">Σ</mml:mi> <mml:mn>1</mml:mn> <mml:mo>+</mml:mo> </mml:msubsup> <mml:mtext> </mml:mtext> <mml:mo fence="false" stretchy="false">|</mml:mo> <mml:mi>v</mml:mi> <mml:mo>=</mml:mo> <mml:mn>22</mml:mn> <mml:mo fence="false" stretchy="false">⟩</mml:mo> <mml:mo>∼</mml:mo> <mml:msup> <mml:mi>b</mml:mi> <mml:mn>3</mml:mn> </mml:msup> <mml:msub> <mml:mi mathvariant="normal">Π</mml:mi> <mml:mn>1</mml:mn> </mml:msub> <mml:mtext> </mml:mtext> <mml:mo fence="false" stretchy="false">|</mml:mo> <mml:mi>v</mml:mi> <mml:mo>=</mml:mo> <mml:mn>54</mml:mn> <mml:mo fence="false" stretchy="false">⟩</mml:mo> </mml:math> state as an efficient bridge for stimulated Raman adiabatic passage. We demonstrate transfer into the NaCs ground state with an efficiency of up to 88(4)%. Highly efficient transfer is critical for the realization of many-body quantum phases of strongly dipolar NaCs molecules and high fidelity detection of single molecules, for example, in spin physics experiments in optical lattices and quantum information experiments in optical tweezer arrays.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Other design · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.671
Threshold uncertainty score0.667

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.016
GPT teacher head0.249
Teacher spread0.233 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designOther design
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations11
Published2023
Admission routes1
Has abstractyes

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