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Record W4380788350 · doi:10.5194/amt-16-3027-2023

Vertical information of CO from TROPOMI total column measurements in context of the CAMS-IFS data assimilation scheme

2023· article· en· W4380788350 on OpenAlexaboutno aff
Tobias Borsdorff, T. Campos, Natalie Kille, Kyle J. Zarzana, Rainer Volkamer, Jochen Landgraf

Bibliographic record

VenueAtmospheric measurement techniques · 2023
Typearticle
Languageen
FieldEnvironmental Science
TopicAtmospheric and Environmental Gas Dynamics
Canadian institutionsnot available
FundersNederlandse Organisatie voor Wetenschappelijk OnderzoekNational Science Foundation
KeywordsEnvironmental scienceTroposphereTrace gasContext (archaeology)AerosolData assimilationRemote sensingMeteorologyPlumeAtmosphere (unit)SCIAMACHYAtmospheric sciencesGeologyGeography

Abstract

fetched live from OpenAlex

Abstract. Since 2017 the Tropospheric Monitoring Instrument (TROPOMI) on board ESA's Copernicus Sentinel-5 satellite (S5-P) has provided the operational carbon monoxide (CO) data product with daily global coverage on a spatial resolution of 5.5×7 km2. The European Centre for Medium-Range Weather Forecasts (ECMWF) plans to assimilate the retrieved total columns and the corresponding vertical sensitivities in the Copernicus Atmosphere Monitoring Service Integrated Forecasting System (CAMS-IFS) to improve forecasts of the atmospheric chemical composition. The TROPOMI data will primarily constrain the vertical integrated CO field of CAMS-IFS but to a lesser extent also its vertical CO distribution. For clear-sky conditions, the vertical sensitivity of the TROPOMI CO data product is useful throughout the atmosphere, but for cloudy scenes it varies due to cloud shielding and light scattering. To assess the profile information, we deploy an a posteriori profile retrieval that combines an ensemble of TROPOMI CO column retrievals with different vertical sensitivities to obtain a vertical CO profile that is then a representative average for the chosen spatial and temporal domain. We demonstrate the approach on three CO pollution cases. For the so-called “Rabbit Foot Fire” in Idaho on 12 August 2018, we estimate a CO profile showing the pollution at an altitude of about 5 km in good agreement with airborne in situ measurements of the Biomass Burning Flux Measurements of Trace Gases and Aerosol (BB-FLUX) field campaign. The distinct CO enhancement in a plume aloft (length =212 km, width =34 km), decoupled from the ground, is sensed by TROPOMI but is not present in the CAMS-IFS model. For a large-scale event, we analyzed the CO pollution from Siberian wildfires that took place from 14 to 17 August 2018. The TROPOMI data estimate the height of the pollution plume over Canada at 7 km in agreement with CAMS-IFS. However, CAMS-IFS underestimates the enhanced CO vertical column densities sensed by TROPOMI within the plume by more than 100 ppb. Finally, we study the seasonal biomass burning in the Amazon. During the burning season the CO profile retrieved from the TROPOMI measurements (1–15 August 2019) agrees well with the one of CAMS-IFS with a similar vertical shape between ground and 14 km altitude. Hence, our results indicate that assimilating TROPOMI CO retrieval with different vertical sensitivities (e.g., under clear-sky and cloudy conditions) provides information about the vertical distribution of CO.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.050
Threshold uncertainty score0.669

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0010.001
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.041
GPT teacher head0.248
Teacher spread0.207 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations10
Published2023
Admission routes1
Has abstractyes

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