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Record W4381378647 · doi:10.26434/chemrxiv-2023-sn90q

Shedding Light on the Stakeholders' Perspectives for Carbon Capture

2023· preprint· en· W4381378647 on OpenAlex
Charithea Charalambous, Elias Moubarak, Johannes Schilling, Eva Sánchez Fernández, Jinyu Wang, Laura Herraiz, Fergus Mcilwaine, Kevin Maik Jablonka, Seyed Mohamad Moosavi, Joren Van Herck, Georges Mouchaham, Christian Serre, André Bardow, Berend Smit, Susana García

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueChemRxiv · 2023
Typepreprint
Languageen
FieldEngineering
TopicCarbon Dioxide Capture Technologies
Canadian institutionsUniversity of Toronto
FundersBundesamt für EnergieU.S. Department of EnergyNatural Environment Research CouncilNorges ForskningsrådUK Research and InnovationEngineering and Physical Sciences Research Council
KeywordsGreenhouse gasProcess (computing)Work (physics)Scale (ratio)Computer scienceCarbon capture and storage (timeline)Process managementEmerging technologiesSystems engineeringEnvironmental economicsRisk analysis (engineering)Management scienceBusinessEngineeringClimate changeEconomics

Abstract

fetched live from OpenAlex

Reducing CO2 emissions requires urgently deploying large-scale carbon capture technologies, amongst other strategies. The quest for optimum technologies is a multi-objective problem involving various stakeholders. Today's research of these technologies follows a sequential approach, with chemists focusing first on material design and engineers subsequently seeking the optimal process. Eventually, this combination of materials and processes operates at a scale that significantly impacts the economy and the environment. Understanding these impacts requires analyzing factors such as greenhouse gas emissions over the lifetime of the capture plant, which now constitutes one of the final steps. In this work, we present the PrISMa (Process-Informed design of tailor-made Sorbent Materials) platform, which seamlessly connects materials, process design, techno-economics, and life-cycle assessment. We compare over sixty case studies in which CO2 is captured from different sources in five world regions with different technologies. These studies illustrate how the platform simultaneously informs all stakeholders: identifying the cheapest technology and optimal process configuration, revealing the molecular characteristics of top-performing materials, determining the best locations, and informing on environmental impacts, co-benefits, and trade-offs. Our platform brings together all stakeholders at an early stage of research, which is essential to accelerate innovations at a time this is most needed.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.580
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.045
GPT teacher head0.242
Teacher spread0.197 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it