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Record W4382653101 · doi:10.1002/9781119678496.ch11

Laser Diode Thermal Desorption‐Mass Spectrometry (LDTD‐MS)

2023· other· en· W4382653101 on OpenAlexaff
Pierre Picard, Sylvain Letarte, Jonathan Rochon, Réal Paquin

Bibliographic record

Venuenot available
Typeother
Languageen
FieldChemistry
TopicSpectroscopy and Laser Applications
Canadian institutionsUniversité LavalPhytronix (Canada)
Fundersnot available
KeywordsComputer scienceSample (material)LaserSample preparationField (mathematics)Instrumentation (computer programming)Mass spectrometryProcess (computing)Thermal desorptionProcess engineeringThroughputDiodeNanotechnologyMaterials scienceDesorptionEngineeringChemistryOptoelectronicsPhysicsChromatographyTelecommunicationsMathematicsOptics

Abstract

fetched live from OpenAlex

High-throughput analysis is a necessary concept to optimize the drug development process. LDTD-MS/MS is a powerful tool in this environment as it combines the sensitivity and speed required for this type of application. This chapter is intended to present several aspects of laser diode thermal desorption technology. The goal is for the reader to understand the technology, its advantages and limitations, the strategies to be used for their applications, and to make the best use of it. The chapter begins with a review of the instrumentation and the theory behind it. Then, the different approaches to sample preparation are presented to the reader. As the sample must be dried before being analyzed, the preparation differs from what is normally done in LC-MS/MS. The preparation techniques for LDTD-MS/MS analysis are adapted according to the matrices and applications. In order to give an overview of the field of application of the technology, several applications described in the literature are discussed. Finally, the advantages of this technique as well as its limitations are also discussed at the end of the chapter.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesInsufficient payload (model declined to judge)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: Not applicable
GenreCandidate signal: Other · Consensus signal: Other
Teacher disagreement score0.436
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0010.000
Insufficient payload (model declined to judge)0.4510.015

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.255
Teacher spread0.244 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; both teacher heads agree on what is shown here.

Study designNot applicable
Domainnot available
GenreOther

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2023
Admission routes1
Has abstractyes

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