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Synergistic Effect of Acarbose–Chlorogenic Acid on α-Glucosidase Inhibition: Kinetics and Interaction Studies Reveal Mixed-Type Inhibition and Denaturant Effect of Chlorogenic Acid

2023· article· en· W4382932180 on OpenAlexafffund
Raliat O. Abioye, O. Charles Nwamba, Ogadimma D. Okagu, Chibuike C. Udenigwe

Bibliographic record

VenueACS Food Science & Technology · 2023
Typearticle
Languageen
FieldMedicine
TopicNatural Antidiabetic Agents Studies
Canadian institutionsUniversity of Ottawa
FundersNatural Sciences and Engineering Research Council of CanadaUniversity of Ottawa
KeywordsAcarboseChlorogenic acidNon-competitive inhibitionChemistryNutraceuticalBiochemistryKineticsPharmacologyEnzymeFood scienceBiology

Abstract

fetched live from OpenAlex

The α-glucosidase inhibitory mechanism of chlorogenic acid was evaluated in the presence of an antidiabetic drug, acarbose. Enzyme kinetics showed the mode of inhibition of the chlorogenic acid–acarbose combination to be either mixed inhibition (competitive and noncompetitive inhibition) or solely competitive inhibition, depending on the dominating inhibitor in the dual system. Despite weaker inhibition by chlorogenic acid, supplementation with acarbose exhibited a synergistic effect on α-glucosidase inhibition, with acarbose equivalent activity exceeding the concentration of acarbose present. Fluorescence quenching studies indicated an increased affinity of chlorogenic acid in the presence of acarbose with an effective quenching constant increasing from 1.6 ± 0.11 × 10 4 to 3.9 ± 0.32 × 10 4 M –1 . Furthermore, acarbose did not affect the static binding mode or the number of chlorogenic acid bound per α-glucosidase molecule. This chlorogenic acid–acarbose dual inhibition system highlights the potential for antidiabetic nutraceuticals as adjuvant therapy for acarbose-based treatments in diabetes management and, to a broader extent, reveals that nutraceuticals can significantly modify or regulate drug-disease state dynamics.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.017
GPT teacher head0.302
Teacher spread0.285 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations14
Published2023
Admission routes2
Has abstractyes

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Same venueACS Food Science & TechnologySame topicNatural Antidiabetic Agents StudiesFrench-language works237,207