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Record W4384389999 · doi:10.48550/arxiv.2307.06486

Absence of $3a_0$ Charge Density Wave Order in the Infinite Layer Nickelates

2023· preprint· en· W4384389999 on OpenAlexafffund
C. T. Parzyck, Naman Gupta, Y. Wu, V. Anil, Lopa Bhatt, M. Bouliane, Rantong Gong, Benjamin Gregory, Aileen Luo, Ronny Sutarto, Feizhou He, Yi‐De Chuang, Tao Zhou, G. Herranz, Lena F. Kourkoutis, Andrej Singer, Darrell G. Schlom, D. G. Hawthorn, K. M. Shen

Bibliographic record

VenuearXiv (Cornell University) · 2023
Typepreprint
Languageen
FieldMaterials Science
TopicMagnetic and transport properties of perovskites and related materials
Canadian institutionsCanadian Light Source (Canada)University of Waterloo
FundersArgonne National LaboratoryBasic Energy SciencesNatural Sciences and Engineering Research Council of CanadaCanadian Institutes of Health ResearchGordon and Betty Moore FoundationU.S. Department of EnergyDivision of Materials ResearchOffice of ScienceCanadian Light SourceNational Science Foundation
KeywordsCuprateCondensed matter physicsSuperconductivityCharge density waveSuperlatticeCharge (physics)PhysicsScatteringOrder (exchange)Charge densityPhase (matter)Quantum mechanics

Abstract

fetched live from OpenAlex

A hallmark of many unconventional superconductors is the presence of many-body interactions which give rise to broken symmetry states intertwined with superconductivity. Recent resonant soft x-ray scattering experiments report commensurate $3a_0$ charge density wave order in the infinite layer nickelates, which has important implications regarding the universal interplay between charge order and superconductivity in both the cuprates and nickelates. Here, we present x-ray scattering and spectroscopy measurements on a series of NdNiO$_{2+x}$ samples which reveal that the signatures of charge density wave order are absent in fully reduced, single-phase NdNiO$_2$. The $3a_0$ superlattice peak instead originates from a partially reduced impurity phase where excess apical oxygens form ordered rows with 3 unit cell periodicity. The absence of any observable charge density wave order in NdNiO$_2$ highlights a crucial difference between the phase diagrams of the cuprate and nickelate superconductors.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.004

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.001
Scholarly communication0.0010.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.091
GPT teacher head0.190
Teacher spread0.099 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations2
Published2023
Admission routes2
Has abstractyes

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Same venuearXiv (Cornell University)Same topicMagnetic and transport properties of perovskites and related materialsFrench-language works237,207