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Record W4385272961 · doi:10.1098/rsbm.2023.0002

Hugh Allen Oliver Hill. 23 May 1937—30 July 2021

2023· article· en· W4385272961 on OpenAlexfundno aff
Peter J. Sadler FRS

Bibliographic record

VenueBiographical Memoirs of Fellows of the Royal Society · 2023
Typearticle
Languageen
FieldChemistry
TopicElectrochemical Analysis and Applications
Canadian institutionsnot available
FundersQueen's UniversityQueen's University Belfast
KeywordsNanotechnologyFerroceneElectron transferGlucose oxidaseChemistryElectrodeElectrochemistryMaterials scienceBiosensorPhysical chemistry

Abstract

fetched live from OpenAlex

Allen Hill was one of the pioneers who established bioinorganic chemistry as an academic discipline. His transition from early research in organic chemistry to the biocoordination chemistry of metals led to the invention of the glucose electrode, which provided for the first time an electronic (amperometric) determination of glucose levels in blood. He guided its commercialization and subsequent use by millions of diabetics worldwide. He and his co-workers made crucial discoveries of how small molecules, especially ferrocene derivatives, can mediate electron transfer from enzymes such as glucose oxidase to electrode surfaces. He used scanning probe microscopy to reveal molecular interactions between proteins and electrode surfaces, and even resolve bound metals at near-atomic resolution. His studies of the biological redox properties and interactions of metals involved not only electrochemical methods, but also nuclear magnetic resonance, electron paramagnetic resonance and Mössbauer spectroscopies. He enjoyed the power of creativity and discovery, and was an exceptional mentor for early career researchers, with an ability to think broadly across the sciences and medicine. He gave devoted service to his college and the University of Oxford, was highly respected internationally and valued greatly the support and encouragement of his own family.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: Not applicable
GenreCandidate signal: Other · Consensus signal: Other
Teacher disagreement score0.342
Threshold uncertainty score0.939

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.000
Science and technology studies0.0010.001
Scholarly communication0.0020.001
Open science0.0010.002
Research integrity0.0020.002
Insufficient payload (model declined to judge)0.3420.257

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.229
Teacher spread0.220 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

Study designNot applicable
Domainnot available
GenreOther

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2023
Admission routes1
Has abstractyes

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Same venueBiographical Memoirs of Fellows of the Royal SocietySame topicElectrochemical Analysis and ApplicationsFrench-language works237,207