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Multi-objective Optimization of a Novel Hybrid Structure for Co-generation of Ammonium Bicarbonate, Formic Acid, and Methanol with Net-Zero Carbon Emissions

2023· article· en· W4385304464 on OpenAlexafffund
Bahram Ghorbani, Sohrab Zendehboudi, Mohammad Hossein Monajati Saharkhiz, Zahra Alizadeh Afrouzi, Omid Mohammadzadeh, Ali Elkamel

Bibliographic record

VenueEnergy & Fuels · 2023
Typearticle
Languageen
FieldEngineering
TopicCarbon Dioxide Capture Technologies
Canadian institutionsUniversity of WaterlooMemorial University of Newfoundland
FundersNatural Sciences and Engineering Research Council of CanadaMemorial University of NewfoundlandMitacs
KeywordsFormic acidChemistryMethanolAmmonium bicarbonateProcess engineeringExergyFlue gasProcess integrationEnvironmental scienceChromatographyOrganic chemistryEngineering

Abstract

fetched live from OpenAlex

Chemical storage of hydrogen, originated from renewable energy, is one of the most efficient and reliable methods to absorb carbon dioxide (CO 2 ) and easily transport large-scale energy to remote areas. In this study, a novel integration of an electro-thermochemical process with industrial flue gas thermal energy and wind turbines is proposed to absorb CO 2 and store chemically hydrogen in the form of methanol, formic acid, and ammonium bicarbonate. The proposed hybrid structure includes a post-combustion CO 2 capture technology, a copper–chlorine thermochemical process, and several ammonium bicarbonate, formic acid, and methanol production cycles. The proposed configuration produces 2597 kg/h methanol, 5270 kg/h ammonium bicarbonate, and 833.3 kg/h formic acid. The energy and exergy efficiencies of the proposed layout are computed at 63.68 and 66.82%, respectively. The exergy analysis depicts that three processes of electro-thermochemical, methanol production, and post-combustion CO 2 capture have the greatest destructed exergy contributions among other subsections to the amounts of 40.85, 30.16, and 7.97%, respectively. The verification, validation, and sensitivity analyses, along with a multi-objective optimization protocol (i.e., a hybrid neural network and a genetic algorithm), are also used to evaluate the proposed system. The objective functions, decision variables, and constraints for the optimization phase are determined through sensitivity analysis. Several multi-criteria decision evaluation methods are employed to prioritize and choose the optimal point from the Pareto set. The electrical power supplied from the wind turbines as well as the auxiliary power supply, and the energy and exergy efficiencies calculated based on the TOPSIS/LINAMP techniques are 9.90 MW, 89.23, and 67.27%, respectively. In addition, the power consumption, energy, and exergy efficiencies at the optimal operating condition, calculated using the Bellman–Zadeh approach, are 9.673 MW, 83.26, and 67.19%, respectively.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.092
Threshold uncertainty score0.723

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.018
GPT teacher head0.232
Teacher spread0.214 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations25
Published2023
Admission routes2
Has abstractyes

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