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Record W4385428527 · doi:10.1038/s41545-023-00271-9

Facile morphological tuning of thin film composite membranes for enhanced desalination performance

2023· article· en· W4385428527 on OpenAlexfundno aff
Shabin Mohammed, Jamaliah Aburabie, Raed Hashaikeh

Bibliographic record

Venuenpj Clean Water · 2023
Typearticle
Languageen
FieldEnvironmental Science
TopicMembrane Separation Technologies
Canadian institutionsnot available
FundersTamkeenYork UniversityNew York University Abu Dhabi
KeywordsMembraneMaterials scienceInterfacial polymerizationPolyamideChemical engineeringThin-film composite membraneNanofiltrationDesalinationLayer (electronics)Composite numberMonomerPolymer chemistryComposite materialReverse osmosisPolymerChemistry

Abstract

fetched live from OpenAlex

Abstract Polyamide (PA) membranes with a thin selective layer have been widely investigated for desalination and water treatment. Several modifications have been proposed over the years to tailor the morphology of such thin film composite (TFC) membranes by altering the support and/or selective layers to achieve superior performance. In this study, a facile approach towards fabricating a highly wrinkled selective layer has been demonstrated through bio-inspired modification of the support layer with Y-type zeolites. Results showed that incorporating zeolites in a smaller dimension (200 nm) produced by a unique ball milling technique is favorable for a defect-free selective layer in comparison to larger commercial zeolites. PA membranes formed by the interfacial polymerization (IP) of Piperazine (PIP) and 1,3,5-Benzenetricarbonyl trichloride (TMC) revealed highly wrinkled morphology due to the presence of zeolites in the TFC interlayer. At optimum fabrication conditions, the membrane exhibited a fast transport of 22.5 ± 2.2 Lm-2h-1bar-1 with a salt rejection of 48.6, 91.3, 99.1, and 99.5% for NaCl, MgCl2, MgSO4, and Na2SO4, respectively. Besides the unique preparation of zeolites in smaller dimensions, the novelty of this study lies in the facile membrane pretreatment before IP to achieve wrinkled PA membranes for enhanced nanofiltration performance.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.026
GPT teacher head0.253
Teacher spread0.228 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations33
Published2023
Admission routes1
Has abstractyes

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