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Record W4385839282 · doi:10.1021/acs.iecr.3c01492

Electrospray Preparation of Robust Aramid Nanofiber Microbead Adsorbents for Wastewater Treatment

2023· article· en· W4385839282 on OpenAlexaff
Jie Yang, Yinghui Zhao, Wentao Liu, Wenshuai Yang, Sheng Chen, Bin Yan

Bibliographic record

VenueIndustrial & Engineering Chemistry Research · 2023
Typearticle
Languageen
FieldMaterials Science
TopicSupercapacitor Materials and Fabrication
Canadian institutionsUniversity of Alberta
FundersDepartment of Science and Technology of Sichuan ProvinceNational Natural Science Foundation of China
KeywordsAdsorptionMicrobead (research)Chemical engineeringNanofiberMaterials scienceStackingDesorptionPorosityNanotechnologyChromatographyChemistryOrganic chemistryComposite material

Abstract

fetched live from OpenAlex

Adsorption is one of the promising techniques for effectively removing dyes from wastewater due to its low cost and high efficiency. However, most reported adsorbents still suffer from low adsorption capacity and stability under harsh conditions, which severely limit their practical application. Herein, we report a novel method to prepare robust aramid nanofiber (ANF) microbead adsorbents using electrospraying technology and solvent replacement method. The structure of the ANF microbeads can be easily manipulated by changing the coagulation baths, thus achieving fabricated ANF microbeads with a uniform and highly porous microstructure. The as-prepared ANF microbeads show high removal efficiency toward methylene blue (MB) with a maximum adsorption capacity of up to 267 mg/g, which can be attributed to the strong π–π stacking, hydrogen bonding, and electrostatic attraction between MB and the microbeads. Moreover, ANF microbeads show outstanding stability within a wide pH range (from 2 to 12) with an MB removal efficiency over 90% even after five adsorption–desorption cycles at pH = 12. Additionally, the ANF microbeads can maintain their structure integrity after the adsorption process and can be easily separated from the solution by static sedimentation because of their robust structure. This work provides a new strategy to design robust microbeads with excellent adsorption performance and stability, demonstrating their great potential in various environmental engineering applications.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.117
GPT teacher head0.347
Teacher spread0.231 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations6
Published2023
Admission routes1
Has abstractyes

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