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Broadband Sensing with High-Performance Non-Fullerene Acceptor-Based Organic Photodetectors

2023· article· en· W4386214608 on OpenAlexaff
Hossein Anabestani, Sharmistha Bhadra

Bibliographic record

Venuenot available
Typearticle
Languageen
FieldEngineering
TopicOrganic Electronics and Photovoltaics
Canadian institutionsMcGill University
Fundersnot available
KeywordsPhotodetectorMaterials scienceFullereneAcceptorOptoelectronicsAbsorption (acoustics)BroadbandActive layerLayer (electronics)OpticsNanotechnologyChemistryOrganic chemistryThin-film transistorPhysics

Abstract

fetched live from OpenAlex

Organic photodetectors (OPDs) are promising optoelectronic technologies due to their low cost, versatility, and ease of processing. OPDs based on conventional fullerene acceptors show narrow absorption window, which limits performance of the OPDs. In this work we present fabrication and characterization of non-fullerene acceptor (NFA), 3,9-bis(2-methylene-((3-(1,1-dicyanomethylene)-6,7-difluoro)-indanone))-5,5,11,11-tetrakis(4-hexylphenyl)-dithieno[2,3-d:2′,3′-d']-s indaceno[1,2-b:5,6-b']dithiophene (IT-4F) based organic photodetectors to have broadband sensing. Two types of NFA based OPDs are fabricated. For the first type only IT-4F is used as an acceptor material, whereas for the second type IT-4F mixed with a fullerene acceptor, [6, 6]-Phenyl-C61-butyric acid methyl ester (PC61BM) is used as an acceptor layer. Although both types of NFA based photodetectors show broadband sensing, the second type exhibits better charge transportation in the active layer than the first type, indicating their potential for broadband light sensing.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0010.001
Open science0.0000.000
Research integrity0.0010.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.175
Teacher spread0.170 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2023
Admission routes1
Has abstractyes

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