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Record W4386221024 · doi:10.3390/coatings13091508

Features of Tribooxidation of the High-Entropy Coating (AlCrZrTiTa)N during Dry High-Speed Cutting

2023· article· en· W4386221024 on OpenAlexaff
А. И. Ковалев, Dmitry Wainstein, Egor Konovalov, Vladimir Vakhrushev, German Fox‐Rabinovich, Michael Fox-Rabinovich, S. A. Dmitrievskii, Alexandr Tomchuk

Bibliographic record

VenueCoatings · 2023
Typearticle
Languageen
FieldEngineering
TopicHigh Entropy Alloys Studies
Canadian institutionsMcMaster University
FundersRussian Science Foundation
KeywordsMaterials scienceAmorphous solidNanocrystalline materialCoatingMicrostructureNanoindentationPhysical vapor depositionElastic modulusRaman spectroscopyComposite materialCrystallographyNanotechnologyChemistry

Abstract

fetched live from OpenAlex

The high-entropy PVD coating (AlCrZrTiTa)N, characterized by its high hardness (50–60 GPa), elastic modulus above 300 MPa, and high heat resistance up to 1300 °C, is used for coating cutting tools operating under extreme metalworking conditions. The nanostructured monolayer 3 μm PVD coating was deposited on cutting plates in the hybrid arc deposition PVD coater. The coating had an amorphous nanocrystalline microstructure with a grain size of about 10–50 nm. The samples of SS 304 steel were investigated during dry high-speed (600 m/min) cutting. Raman spectroscopy was used to study the formation of tribooxides on the tool surface at the running-in stage of the cutting. After 130 m of cutting, Cr2O3 oxide appears on the wear surface while other elements are bound with N atoms. When the cutting length is increased to up to 260 m, oxide Al2O3 · ZrO2 (mullite) and amorphous oxides TaO2 and CrO2 are formed. The method EELFS made it possible to determine the amorphous nanocrystalline structure of triboceramics based on CrO2 and Al2O3 · ZrO2. The nearest atomic surrounding of Cr-Cr, O-O, and Cr-O and their subsequent comparison with the available literature data allow us to calculate the equilibrium lattice constants of the CrO2 unit cell, which are equal to (a, b) = 4.3754 Å and c = 0.5927. The triboceramic films on the base of non-equilibrium mullite Al2O3·ZrO2 have an amorphous structure. In the first coordination sphere, the interatomic distances of Zr-O and Al-O were 1.79 and 1.89 Å. An accelerated adaptive reaction to extreme external stimuli, at the very beginning of the running-in stage, is established. The tribological adaptability of the high-entropy ultra-fine amorphous nanocrystalline coating under extremely loaded dry high-speed cutting is based on non-equilibrium phenomena: the partial oxidation of fragments of the nitride and dynamic formation of protective tribooxides, which have a good thermal barrier and frictional properties. These factors interact synergistically and determine the life of the cutting tool.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.191
Threshold uncertainty score0.664

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.207
Teacher spread0.200 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations6
Published2023
Admission routes1
Has abstractyes

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