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Record W4386249195 · doi:10.1021/acsnano.3c04420

Quantitation of Circulating <i>Mycobacterium tuberculosis</i> Antigens by Nanopore Biosensing in Children Evaluated for Pulmonary Tuberculosis in South Africa

2023· article· en· W4386249195 on OpenAlexaff
Xiaoqin Wang, Xiaojun Wei, Marieke M. van der Zalm, Zehui Zhang, Nandhini Subramanian, Anne‐Marie Demers, Elisabetta Walters, Anneke C. Hesseling, Chang Liu

Bibliographic record

VenueACS Nano · 2023
Typearticle
Languageen
FieldEngineering
TopicNanopore and Nanochannel Transport Studies
Canadian institutionsUniversité de MontréalCentre Hospitalier Universitaire Sainte-Justine
FundersEuropean and Developing Countries Clinical Trials PartnershipDivision of Chemical, Bioengineering, Environmental, and Transport SystemsFogarty International CenterFaculty of Medicine and Health, University of SydneyHarry Crossley FoundationNational Institute of Allergy and Infectious DiseasesMedical Research CouncilSouth African Medical Research CouncilHorizon 2020 Framework ProgrammeNational Research FoundationEuropean CommissionNational Institutes of HealthUniversiteit StellenboschNational Science Foundation
KeywordsNanoporeTuberculosisMycobacterium tuberculosisAnalyteAntigenBiosensorNanopore sequencingNanotechnologyMycobacterium tuberculosis complexGold standard (test)Clinical diagnosisDiseaseMedicineVirologyImmunologyBiologyMaterials scienceChemistryInternal medicineIntensive care medicinePathologyChromatographyGenome

Abstract

fetched live from OpenAlex

Nanopore sensing of proteomic biomarkers lacks accuracy due to the ultralow abundance of targets, a wide variety of interferents in clinical samples, and the mismatch between pore and analyte sizes. By converting antigens to DNA probes via click chemistry and quantifying their characteristic signals, we show a nanopore assay with several amplification mechanisms to achieve an attomolar level limit of detection that enables quantitation of the circulating Mycobacterium tuberculosis ( Mtb ) antigen ESAT-6/CFP-10 complex in human serum. The assay’s nonsputum-based feature and low-volume sample requirements make it particularly well-suited for detecting pediatric tuberculosis (TB) disease, where establishing an accurate diagnosis is greatly complicated by the paucibacillary nature of respiratory secretions, nonspecific symptoms, and challenges with sample collection. In the clinical assessment, the assay was applied to analyze ESAT-6/CFP-10 levels in serum samples collected during baseline investigation for TB in 75 children, aged 0–12 years, enrolled in a diagnostic study conducted in Cape Town, South Africa. This nanopore assay showed superior sensitivity in children with confirmed TB (94.4%) compared to clinical “gold standard” diagnostic technologies (Xpert MTB/RIF 44.4% and Mtb culture 72.2%) and filled the diagnostic gap for children with unconfirmed TB, where these traditional technologies fell short. We envision that, in combination with automated sample processing and portable nanopore devices, this methodology will offer a powerful tool to support the diagnosis of pulmonary TB in children.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.293
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.002
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.017
GPT teacher head0.233
Teacher spread0.217 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations15
Published2023
Admission routes1
Has abstractyes

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