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Record W4386290421 · doi:10.1002/cjce.25074

Preparation of <scp>ZIF</scp> ‐8—Pebax 1657 nanocomposite membranes for <i>n</i> ‐hexane/nitrogen separation as a representative of gasoline vapour recovery

2023· article· en· W4386290421 on OpenAlexvenueno aff
Shabnam Lorvand, Omid Bakhtiari

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2023
Typearticle
Languageen
FieldEngineering
TopicMembrane Separation and Gas Transport
Canadian institutionsnot available
Fundersnot available
KeywordsPermeationMembraneHexaneNanocompositeFourier transform infrared spectroscopyChemical engineeringMaterials scienceSelectivityBarrerNitrogenChromatographyChemistryOrganic chemistryComposite materialCatalysis

Abstract

fetched live from OpenAlex

Abstract Gasoline vapour emission is hazardous to both human health and the ecosystem and also results in capital loss, altogether revealing the necessity of its recovery. Some ZIF‐8–Pebax flat nanocomposite membranes were fabricated by the method of solution casting and used for gasoline vapour recovery as represented by n ‐hexane vapour/nitrogen separation. Microporous ZIF‐8 nanoparticles were synthesized and characterized by Fourier transform infrared (FTIR) and Brunauer–Emmett–Teller (BET) analysis. BET results revealed specific surface area, total volume, and average pore diameter of 940.8 m 2 · g −1 , 0.36 cm 3 · g −1 , and 1.54 nm, respectively. Pure nitrogen and n ‐hexane vapour/nitrogen gas mixture permeabilities were measured through the membranes. There was a decline in both permeation rate and selectivity up to 5.0 wt.% of ZIF‐8 loading and the next increment at their higher loadings to considerably more values that the pristine membrane. The maximum n ‐hexane vapour permeability and selectivity at 10.0 wt.% loading of ZIF‐8 nanoparticles, the feed flow rate of 173 mL · min −1 , and permeate side pressure of −200 mbar were observed as 280.1 Barrer and 106.7, respectively, revealing 60.0% and 36.9% improvements compared with those of the pristine Pebax membrane. Observed 86%–92% n ‐hexane vapour recovery approves the successful application of the ZIF‐8–Pebax nanocomposite membranes for n ‐hexane/nitrogen separation. The long‐term separation performance of 5.0 wt.% ZIF‐8 loaded nanocomposite membrane was improved by 76.5% compared with that of the pristine Pebax membrane.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.426
Threshold uncertainty score0.624

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.256
Teacher spread0.245 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations3
Published2023
Admission routes1
Has abstractyes

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