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Record W4386414876 · doi:10.1002/adma.202305238

Buried‐Metal‐Grid Electrodes for Efficient Parallel‐Connected Perovskite Solar Cells

2023· article· en· W4386414876 on OpenAlexaff
Lei Li, Peng Chen, Rui Su, Hongyu Xu, Qiuyang Li, Qixuan Zhong, Haoming Yan, Xiaoyu Yang, Juntao Hu, Shunde Li, Tianyu Huang, Yun Xiao, Bin Liu, Yongqiang Ji, Dengke Wang, Huiliang Sun, Xugang Guo, Zheng‐Hong Lu, Henry J. Snaith, Qihuang Gong, Lichen Zhao, Rui Zhu

Bibliographic record

VenueAdvanced Materials · 2023
Typearticle
Languageen
FieldEngineering
TopicPerovskite Materials and Applications
Canadian institutionsUniversity of Toronto
FundersSongshan Lake Materials LaboratoryNational Key Research and Development Program of ChinaEngineering and Physical Sciences Research CouncilChina Oxford Scholarship FundShenzhen Science and Technology Innovation ProgramBeijing Nova ProgramNatural Science Foundation of Beijing MunicipalityChina Postdoctoral Science FoundationNational Natural Science Foundation of China
KeywordsMaterials scienceIndium tin oxideElectrodeSheet resistanceOptoelectronicsEnergy conversion efficiencyPerovskite (structure)Photovoltaic systemFabricationConductivityNanotechnologyThin filmLayer (electronics)Chemical engineeringElectrical engineering

Abstract

fetched live from OpenAlex

Abstract The limited conductivity of existing transparent conducting oxide (TCO) greatly restricts the further performance improvement of perovskite solar cells (PSCs), especially for large‐area devices. Herein, buried‐metal‐grid tin‐doped indium oxide (BMG ITO) electrodes are developed to minimize the power loss caused by the undesirable high sheet resistance of TCOs. By burying 140‐nm‐thick metal grids into ITO using a photolithography technique, the sheet resistance of ITO is reduced from 15.0 to 2.7 Ω sq −1 . The metal step of BMG over ITO has a huge impact on the charge carrier transport in PSCs. The PSCs using BMG ITO with a low metal step deliver power conversion efficiencies (PCEs) significantly better than that of their counterparts with higher metal steps. Moreover, compared with the pristine ITO‐based PSCs, the BMG ITO‐based PSCs show a smaller PCE decrease when scaling up the active area of devices. The parallel‐connected large‐area PSCs with an active area of 102.8 mm 2 reach a PCE of 22.5%. The BMG ITO electrodes are also compatible with the fabrication of inverted‐structure PSCs and organic solar cells. The work demonstrates the great efficacy of improving the conductivity of TCO by BMG and opens up a promising avenue for constructing highly efficient large‐area PSCs.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.064
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.228
Teacher spread0.220 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations9
Published2023
Admission routes1
Has abstractyes

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