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Record W4386492128 · doi:10.1103/physrevb.108.l121106

Anisotropic Seebeck coefficient of <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:msub><mml:mi>Sr</mml:mi><mml:mn>2</mml:mn></mml:msub><mml:msub><mml:mi>RuO</mml:mi><mml:mn>4</mml:mn></mml:msub></mml:mrow></mml:math> in the incoherent regime

2023· article· lv· W4386492128 on OpenAlexaff
Ramzy Daou, S. Hébert, G. Grissonnanche, Elena Hassinger, Louis Taillefer, Haruka Taniguchi, Y. Maeno, Alexandra S. Gibbs, A. P. Mackenzie

Bibliographic record

VenuePhysical review. B./Physical review. B · 2023
Typearticle
Languagelv
FieldPhysics and Astronomy
TopicAdvanced Condensed Matter Physics
Canadian institutionsRegroupement Québécois sur les Matériaux de PointeUniversité de Sherbrooke
FundersJapan Society for the Promotion of Science
KeywordsSeebeck coefficientAnisotropyIsotropyCondensed matter physicsMaterials scienceThermoelectric effectPhysicsThermodynamicsOptics

Abstract

fetched live from OpenAlex

Intuitive entropic interpretations of the thermoelectric effect in metals predict an isotropic Seebeck coefficient at high temperatures in the incoherent regime even in anisotropic metals since entropy is not directional. ${\mathrm{Sr}}_{2}{\mathrm{RuO}}_{4}$ is an enigmatic material known for a wellcharacterized anisotropic normal state and unconventional superconductivity. Recent ab initio transport calculations of ${\mathrm{Sr}}_{2}{\mathrm{RuO}}_{4}$ that include the effect of strong electronic correlations predicted an enhanced high-temperature anisotropy of the Seebeck coefficient at temperatures above 300 K, but experimental evidence is missing. From measurements on clean ${\mathrm{Sr}}_{2}{\mathrm{RuO}}_{4}$ single crystals along both crystallographic directions, we find that the Seebeck coefficient becomes increasingly isotropic upon heating towards room temperature as generally expected. Above 300 K, however, $S$ acquires a new anisotropy which rises up to the highest temperatures measured (750 K), in qualitative agreement with calculations. This is a challenge to entropic interpretations and highlights the lack of an intuitive framework to understand the anisotropy of thermopower at high temperatures.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.002
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Science and technology studies, Scholarly communication, Research integrity, Insufficient payload (model declined to judge)
Consensus categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.919
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0020.002
Meta-epidemiology (narrow)0.0020.003
Meta-epidemiology (broad)0.0010.004
Bibliometrics0.0000.003
Science and technology studies0.0020.002
Scholarly communication0.0010.002
Open science0.0040.003
Research integrity0.0010.003
Insufficient payload (model declined to judge)0.1240.008

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.020
GPT teacher head0.287
Teacher spread0.266 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; both teacher heads agree on what is shown here.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations3
Published2023
Admission routes1
Has abstractyes

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