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Record W4386748404 · doi:10.58837/chula.the.2017.75

Nanocomposite membranes incorporated with graphene oxide for CO2/CH4 separation

2017· dissertation· en· W4386748404 on OpenAlexaff
Nadia Norahim

Bibliographic record

Venuenot available
Typedissertation
Languageen
FieldEngineering
TopicMembrane Separation and Gas Transport
Canadian institutionsInstitute of Particle Physics
FundersChulalongkorn University
KeywordsPermeanceGrapheneMaterials scienceMembraneChemical engineeringOxideNanocompositeGas separationPolymerComposite materialChemistryNanotechnologyPermeationMetallurgy

Abstract

fetched live from OpenAlex

Biogas is an alternative energy produced by anaerobic digestion of organic matter. Generally, raw biogas consists of methane (CH4), carbon dioxide (CO2), few amount of hydrogen sulfide (H2S) and traces of water vapor. Nowadays, upgrading raw biogas is required in order to achieve higher calorific value and meet fuel standard by removal of CO2. In this study, composite membranes of PEG 400/Pebax 1657 blended polymer with graphene oxide (GO) and amine functionalized graphene oxide (Fn-GO) were successfully developed for CO2/CH4 gas separation. The effects of graphene oxide, amine functionalized graphene oxide and PEG 400 additions on CO2/CH4 separation performance were studied in this research. The membrane containing 0.25 wt.% GO in Pebax 1657 showed a better separation factor compared to pristine Pebax 1657 composite membrane by increasing from 12.18 to 42.33. However, CO2 permeance dropped when GO was incorporated in Pebax matrix. PEG 400 was added in Peabax 1657 matrix to increase CO2 permeance and it was found that the composite membrane containing 50 wt.% PEG 400 in polymer matrix with 0.25 wt.% GO showed the good CO2/CH4 separation factor up to 42.81 and also CO2 permeance of 13.07 GPU. With the obtained results, it could be concluded that GO mainly influenced separation factor because GO generated a rigidified interface between the polymer and fillers Moreover, GO also block the pathway for CH4 through membrane resulting to an increased diffusion distance and enhance the separation between CO2 and CH4. Whereas PEG 400 provided a higher CO2 permeance due to a loose chain of Pebax 1657 matrix.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.251
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.262
Teacher spread0.250 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2017
Admission routes1
Has abstractyes

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