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Record W4386781119 · doi:10.26434/chemrxiv-2023-sb6nk

Process-performance of solid sorbents for Direct Air Capture (DAC) of CO2 in optimized temperature-vacuum swing adsorption (TVSA) cycles

2023· preprint· en· W4386781119 on OpenAlexafffund
Bhubesh Murugappan Balasubramaniam, Phuc-Tien Thierry, Samuel Lethier, Véronique Pugnet, Philip L. Llewellyn, Arvind Rajendran

Bibliographic record

VenueChemRxiv · 2023
Typepreprint
Languageen
FieldEngineering
TopicCarbon Dioxide Capture Technologies
Canadian institutionsUniversity of Alberta
FundersAlliance de recherche numérique du CanadaTotalMitacs
KeywordsAdsorptionSorbentSwingMaterials scienceVacuum swing adsorptionProcess engineeringProcess (computing)Unary operationThermodynamicsChemistryPressure swing adsorptionComputer scienceMechanical engineeringEngineeringMathematicsPhysical chemistryPhysics

Abstract

fetched live from OpenAlex

The process performance of five solid sorbents was evaluated for direct air capture (DAC) of CO2 in temperature-vacuum swing adsorption (TVSA) and steam-assisted temperature vacuum swing adsorption (s-TVSA) cycles via detailed process modelling. The unary CO2, H2O and binary CO2-H2O isotherm data, wherever available, were fit to suitable isotherm models and then integrated with the detailed process model. The trade-off between specific energy and CO2 productivity has been studied through rigorous process optimizations. The study shows that thermal energy demand is substantial in comparison to the electrical energy. The role of steam was primarily found to improve the productivity. The range of minimum specific energy values is between 6.25-30.4 MJth/kg CO2, although, for some of the sorbents, the lack of H2O adsorption data impedes reliable calculations. The range of maximum CO2 productivities observed is between 0.01-0.15 TPD of CO2/m3 of sorbent

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.004
Threshold uncertainty score0.009

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.018
GPT teacher head0.256
Teacher spread0.238 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations7
Published2023
Admission routes2
Has abstractyes

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