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Record W4386854064 · doi:10.1149/ma2023-01271762mtgabs

(Invited) Capacitive Deionization (CDI) – an Industrial Research Perspective

2023· article· en· W4386854064 on OpenAlexaff
Prantik Mazumder, Todd StClair, R.J. Bourcier

Bibliographic record

VenueECS Meeting Abstracts · 2023
Typearticle
Languageen
FieldEngineering
TopicMembrane-based Ion Separation Techniques
Canadian institutionsResearch & Development Corporation
Fundersnot available
KeywordsCapacitive deionizationDesalinationReverse osmosisProcess engineeringEnvironmental sciencePopulationMaterials scienceComputer scienceEnvironmental engineeringEngineeringMembraneChemistry

Abstract

fetched live from OpenAlex

As the demand for freshwater keeps increasing due to industrialization and population growth, the world is progressively interested in desalination for sourcing potable water. While membrane-based reverse osmosis (RO) and thermal-based evaporation/distillation are proven technologies for desalination, they are also expensive. Capacitive deionization (CDI) - introduced in the 1970s - where the positive and negative ions are separated by the application of an electric field across pairs of high surface area electrodes, has been considered as a potentially cheaper technology. In the mid-2000s, Corning carried out a research project on developing CDI. The workstreams involved developing novel materials for electrodes, new device architecture, predictive theoretical models at electrode and device scales, and eventually a plant-level cost analysis that connected the electrode and device-level parameters to the final cost of water desalination, in $/gallon, which is the ultimate arbiter for techno-economic feasibility. We made significant progress in: (a) developing thin all-carbon electrodes which were electrochemically inert, highly conductive, and possessed high specific capacitance (F/cc) (b) designing a flow-past device architecture based on stacked planar electrodes with a small footprint (c) developing user-friendly simplified theoretical models, and (d) formulating two high-level figures of merit (FOM), namely, volumetric efficiency (VE) and recovery ratio (RR) – both of which need to be maximized to compete against incumbent technologies such as RO, especially in the high-throughput brackish water market sector. Our prototype achieved an equivalent VE of ~40 kg/ft 3 /day of salt removal. However, the plant-level cost analysis suggested that there is not much room for improving the overall cost structure compared to RO even with such high device level performance for high throughput desalination markets. In this talk we will present our experience with the development of CDI technology. We will cover all aspects of the project - electrode materials development, device architecture, theoretical models, and cost analysis – and will also offer an industrial perspective on CDI technology development, particularly when it comes to competing against well-established and entrenched technologies. We will also highlight how systems-level thinking and analyses are extremely important for such technology assessments and point out that only focusing on lab-scale performance metrics can be misleading.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.554
Threshold uncertainty score0.784

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0020.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.123
GPT teacher head0.355
Teacher spread0.232 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2023
Admission routes1
Has abstractyes

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