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Record W4386962747 · doi:10.1002/cjce.25090

Original synthesis of polyvinyl butyral with a green deep eutectic solvent and a weakly polyacrylic acid from polyvinyl alcohol and the impacts of the chains structures of polyvinyl alcohol

2023· article· en· W4386962747 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

venuePublished in a venue whose home country is Canada.
no affNo Canadian affiliation: this work is invisible to an affiliation-only frame.
No Canadian affiliation. An affiliation-only frame, the usual design, would never have seen this work. It is one of the works that make the case for inverting the frame.

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2023
Typearticle
Languageen
FieldMaterials Science
TopicPolymer Science and PVC
Canadian institutionsnot available
Fundersnot available
KeywordsPolyvinyl alcoholPolyvinyl butyralPolyacrylic acidPolymer chemistryMaterials scienceSolventUltimate tensile strengthPolymerChemical engineeringEutectic systemPolyvinyl acetateOrganic chemistryChemistryComposite materialMicrostructure

Abstract

fetched live from OpenAlex

Abstract In this work, an environmentally‐friendly deep eutectic solvent (DES) was employed as a catalyst to generate polyvinyl butyral (PVB) resins from polyvinyl alcohol (PVA) with a weakly acidic polymer (polyacrylic acid [PAA]) as an emulsifier. Finally, high viscosity PVB resins with molecular weight of 110,000–200,000 g · mol −1 and acetalization degree above 83% were successfully synthesized, which was found to satisfy the requirements for interlayer films between safety glass. Furthermore, it was well proved that the properties of PVB resins immensely depend on the molecular structures of the PVA. The molecular weight of the PVB, independent of alcoholic degrees of the PVA, indicated an upward trend with the increase of the molecular weight of the PVA. As for these four PVBs with high molecular weight, the T g was sensitive to the content of hydroxyl and acetal groups rather than molecular weight, associated with the inter‐ or intra‐molecule hydrogen bond between OH. PVB‐1799 and PVB‐1797 had higher T i and T g than that of PVB‐1788 and PVB‐1795 because the former had low contents of vinyl acetate group (VAc) and alcohol hydroxyl group (VOH). The tensile strength of PVBs was all higher than 30 Mpa, and the elongation at break was about 300% due to their high molecular weights.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.025
Threshold uncertainty score0.979

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.205
Teacher spread0.196 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it