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Record W4387501537 · doi:10.1063/5.0161954

Investigating the effects of operating parameters on the performance of sorption-enhanced membrane reactor for ethanol steam reforming reaction using computational fluid dynamics method

2023· article· en· W4387501537 on OpenAlexaff
Rahman Zeynali, Seyede Sara Khalili, Zahra Pezeshki, Mona Akbari, Hosna Soleymani, Ehsan Samimi-Sohrforozani, Babak Safaei

Bibliographic record

VenuePhysics of Fluids · 2023
Typearticle
Languageen
FieldChemical Engineering
TopicCatalysts for Methane Reforming
Canadian institutionsUniversity of Saskatchewan
Fundersnot available
KeywordsComputational fluid dynamicsSteam reformingSpace velocityMembrane reactorHydrogenThermodynamicsAdsorptionSorptionMembraneChemical engineeringNuclear engineeringChemistryPhysicsHydrogen productionCatalysisOrganic chemistryEngineering

Abstract

fetched live from OpenAlex

In this study, the performance of a sorption-enhanced membrane reactor (SEMR) was examined using a Pd-Ag membrane during ethanol steam reforming (ESR). During this study, simultaneous ESR and CO2 adsorption concept was adopted and computational fluids dynamic (CFD) method (two-dimensional model) was developed to evaluate the SEMR performance during ESR reaction. The employed CFD model for the present study provided information about the molar fractions and pressures of components to analyze driving forces under unsteady state condition. Regarding validation, the experimental data related to the membrane reactor (MR) during ESR reaction showed good agreement with modeling outcomes and the application of adsorption reaction improved MR performance. The SEMR performance was investigated after model validation, and during this step, SEMR and MR were compared. Moreover, the effects of main operating parameters, such as gas hour space velocity (GHSV), reaction pressure, and temperature, were studied to compare the SEMR and MR performance during C2H5OH conversion and hydrogen recovery. CFD modeling results showed that SEMR had better performance and increased the ethanol conversion about 20% (SEMR: 70% and MR: 59%) by temperature enhancement at low pressures compared with the conventional membrane reactor. The relative error between numerical and experimental data obtained was 3% in this study.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.336
Threshold uncertainty score0.554

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.026
GPT teacher head0.287
Teacher spread0.261 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations4
Published2023
Admission routes1
Has abstractyes

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