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CO2 capture in activated pyrolytic coke/metal oxide nanoparticle composites

2023· article· en· W4387538132 on OpenAlexaff
Narmin Noorani, Behrad Barzegar, Abbas Mehrdad, Hassan Aghdasinia, Seyed Jamaleddin Peighambardoust, Hossein Kazemian

Bibliographic record

VenueColloids and Surfaces A Physicochemical and Engineering Aspects · 2023
Typearticle
Languageen
FieldEngineering
TopicCarbon Dioxide Capture Technologies
Canadian institutionsUniversity of Northern British Columbia
Fundersnot available
KeywordsMaterials scienceAdsorptionActivated carbonPyrolytic carbonOxideComposite numberComposite materialChemical engineeringNanoparticleCokeIron oxidePyrolysisNanotechnologyMetallurgyChemistryOrganic chemistry

Abstract

fetched live from OpenAlex

Carbon dioxide (CO 2 ) capture from flue gas is of utmost importance in mitigating greenhouse gas emissions. This study focuses on enhancing the CO 2 adsorption capacity of activated carbon (AC) composites through the incorporation of metal oxides . AC, AC/Fe 3 O 4 , and AC/MgO composites were synthesized and characterized using various analytical techniques including Raman and FTIR spectroscopy , TGA , SEM, EDX , XRD , AFM, BET, and VSM analysis. The CO2 adsorption isotherms of the AC/MgO and AC/Fe 3 O 4 composites were measured at different temperatures and pressures using quartz crystal microbalance (QCM). The Langmuir model was successfully employed to fit the experimental data, with AC/MgO and AC/Fe 3 O 4 exhibiting adsorption capacities of 38.567 mmol g − 1 and 71.963 mmol g − 1 , respectively, at 298.15 K and 5 bar. These results demonstrate the significant enhancement of CO 2 adsorption capacity achieved by incorporating metal oxides into the AC composite structure. Furthermore, the regeneration efficiency of the adsorbents was evaluated through multiple adsorption/desorption cycles, revealing that AC, AC/MgO, and AC/Fe 3 O 4 maintained adsorption capacities of 94.1%, 97.9%, and 96.5%, respectively, after six consecutive cycles. This confirms their stability and reusability under practical conditions. These findings contribute to our understanding of CO 2 capture using activated pyrolytic coke and metal oxide nanoparticle composites, highlighting the promising potential of AC/MgO composites as effective adsorbents for CO 2 capture applications. Further investigation and optimization of composite structures and synthesis methods are warranted to enhance their overall performance and applicability

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.186
Threshold uncertainty score0.960

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.180
Teacher spread0.174 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations20
Published2023
Admission routes1
Has abstractyes

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