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Record W4387703322 · doi:10.1021/acssuschemeng.3c04373

Scale-Dependent Techno-Economic Analysis of CO<sub>2</sub> Capture and Electroreduction to Ethylene

2023· article· en· W4387703322 on OpenAlexafffund
Théo Alerte, Adriana Gaona, Jonathan P. Edwards, Christine M. Gabardo, Colin P. O’Brien, Joshua Wicks, Loann Bonnenfant, Armin Sedighian Rasouli, Daniel Young, Jehad Abed, Luke Kershaw, Yurou Celine Xiao, Amitava Sarkar, Shaffiq A. Jaffer, Moritz W. Schreiber, David Sinton, Heather L. MacLean, Edward H. Sargent

Bibliographic record

VenueACS Sustainable Chemistry & Engineering · 2023
Typearticle
Languageen
FieldEnergy
TopicCO2 Reduction Techniques and Catalysts
Canadian institutionsUniversity of Toronto
FundersNatural Resources CanadaTotalNatural Sciences and Engineering Research Council of CanadaCanada Research Chairs
KeywordsPetrochemicalDownstream (manufacturing)Renewable energyProfitability indexEnvironmental scienceProcess engineeringUpstream (networking)Waste managementProduction (economics)TonneGreenhouse gasElectricityScale (ratio)Environmental engineeringEngineeringBusinessOperations managementEconomics

Abstract

fetched live from OpenAlex

The decarbonization of the chemical industry is essential to mitigate carbon dioxide (CO 2 ) emissions. Ethylene (C 2 H 4 ) is the highest production petrochemical globally. When powered by renewable electricity, the electrochemical conversion of CO 2 to C 2 H 4 offers a promising route to low carbon C 2 H 4 production. We perform a detailed techno-economic assessment (TEA) of the CO 2 reduction reaction (CO 2 RR) process, converting CO 2 from an industrial point source to polymer-grade C 2 H 4 . We pair the CO 2 electrolyzer with industrially mature upstream and downstream separation technologies in an Aspen Plus model. This comprehensive approach enables us to assess the valorization of both gas and liquid byproduct streams at commercial specification and assess the viability of these processes as a function of scale. We demonstrate that a minimum plant size of ∼3,000 tonne C 2 H 4 /year is needed to achieve economies of scale among the upstream and downstream processes. This minimum plant size is ∼200-fold smaller than that of conventional C 2 H 4 plants, coincides with that of typical utility-scale solar installations (∼25 MW), and could enable a more distributed model of chemical production going forward. We further highlight technical and economic enablers that would increase the profitability of the CO 2 RR to C 2 H 4 technology.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: Simulation or modeling
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.004
Threshold uncertainty score0.008

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.003
GPT teacher head0.204
Teacher spread0.201 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations36
Published2023
Admission routes2
Has abstractyes

Explore more

Same venueACS Sustainable Chemistry & EngineeringSame topicCO2 Reduction Techniques and CatalystsFrench-language works237,207