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Record W4387761014 · doi:10.1126/sciadv.adi4966

Potential Lifshitz transition at optimal substitution in nematic pnictide Ba <sub> 1− <i>x</i> </sub> Sr <i> <sub>x</sub> </i> Ni <sub>2</sub> As <sub>2</sub>

2023· article· en· W4387761014 on OpenAlexaff
Dushyant Narayan, Peipei Hao, R. Kurleto, Bryan S. Berggren, A. Garrison Linn, Chris Eckberg, Prathum Saraf, John Collini, Peter Y. Zavalij, Makoto Hashimoto, Dong-Hui Lu, Rafael M. Fernandes, Johnpierre Paglione, D. S. Dessau

Bibliographic record

VenueScience Advances · 2023
Typearticle
Languageen
FieldMaterials Science
TopicIron-based superconductors research
Canadian institutionsCanadian Institute for Advanced Research
FundersSLAC National Accelerator LaboratoryOffice of ScienceBasic Energy SciencesDiamond Light SourceGordon and Betty Moore FoundationU.S. Department of Energy
KeywordsSuperconductivityPnictogenCondensed matter physicsAngle-resolved photoemission spectroscopyLiquid crystalDensity functional theoryTransition temperaturePhotoemission spectroscopyMaterials sciencePhysicsElectronic structureNuclear magnetic resonanceQuantum mechanicsX-ray photoelectron spectroscopy

Abstract

fetched live from OpenAlex

BaNi 2 As 2 is a structural analog of the pnictide superconductor BaFe 2 As 2 , which, like the iron-based superconductors, hosts a variety of ordered phases including charge density waves (CDWs), electronic nematicity, and superconductivity. Upon isovalent Sr substitution on the Ba site, the charge and nematic orders are suppressed, followed by a sixfold enhancement of the superconducting transition temperature ( T c ). To understand the mechanisms responsible for enhancement of T c , we present high-resolution angle-resolved photoemission spectroscopy (ARPES) measurements of the Ba 1− x Sr x Ni 2 As 2 series, which agree well with our density functional theory (DFT) calculations throughout the substitution range. Analysis of our ARPES-validated DFT results indicates a Lifshitz transition and reasonably nested electron and hole Fermi pockets near optimal substitution where T c is maximum. These nested pockets host Ni d xz /d yz orbital compositions, which we associate with the enhancement of nematic fluctuations, revealing unexpected connections to the iron-pnictide superconductors. This gives credence to a scenario in which nematic fluctuations drive an enhanced T c .

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.007
metaresearch head score (Gemma)0.002
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Science and technology studies, Scholarly communication, Insufficient payload (model declined to judge)
Consensus categoriesMeta-epidemiology (narrow), Science and technology studies
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.034
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0070.002
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0020.008
Science and technology studies0.0030.005
Scholarly communication0.0010.009
Open science0.0030.001
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0000.005

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.269
Teacher spread0.256 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; both teacher heads agree on what is shown here.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations8
Published2023
Admission routes1
Has abstractyes

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