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Record W4387816250 · doi:10.1021/acsomega.3c05772

Reduction–Sulfurization Smelting Process of Waste Hydrogenation Catalysts, Automotive Exhaust Purifier Waste Catalysts, and Laterite Nickel Ore

2023· article· en· W4387816250 on OpenAlexaff
Zihao Wang, Haibei Wang, Xiaowu Jie, Xu Zhao, Kristian E. Waters, Derek O. Northwood, Senlin Cui, Hao Ma

Bibliographic record

VenueACS Omega · 2023
Typearticle
Languageen
FieldEngineering
TopicMetal Extraction and Bioleaching
Canadian institutionsUniversity of WindsorMcGill University
FundersNational Key Research and Development Program of China
KeywordsWaste managementLateriteSmeltingNickelCatalysisEnvironmental scienceMetallurgyMaterials scienceChemistryEngineering

Abstract

fetched live from OpenAlex

High Resolution Image Download MS PowerPoint Slide Reduction–sulfurization smelting is an effective method for treating solid hazardous waste and recovering valuable components from them. In this work, a waste hydrogenation catalyst (WHC), an automotive exhaust purifier waste catalyst (AEPWC), a vulcanizer, and laterite nickel ore were mixed, and the reduction smelting behavior of this solid waste was investigated. XRD (X-ray diffractometry), TG-DSC (thermogravimetric/differential scanning calorimetry), SEM-EDS (scanning electron microscopy-energy dispersive spectroscopy), OM (optical microscopy), and ICP-OES (inductively coupled plasma-optical emission spectrometry) methods were used to examine the chemical composition, thermal stability, structure, and morphology, as well as the metal content of the samples. Under the Al 2 O 3 -FeO-SiO 2 ternary slag system, at a smelting temperature of 1450 °C, smelting time of 2 h, mass ratio of coke, pyrite, and CaO to waste catalysts of 16, 25, and 0%, respectively, nickel (Ni) and molybdenum (Mo) recovery reached 91.1 and 92.9%, respectively, where average PGMs (platinum group metals, platinum (Pt), palladium (Pd), rhodium (Rh)) recovery reached 96%, although vanadium (V) recovery was only 25.1%. The characterization of the slag shows that Al, Si, and Fe are mainly bound in the form of chemical compounds, while V is intercalated with ferro- or aluminosilicate, which hinders the reduction and sulfurization of V. A series of tests using reduction smelting without sulfurization were also conducted, after which the Ni, Mo, and V recovery reached 96.8, 96.6, and 89.7%, respectively, while PGMs (Pt, Pd, Rh) recovery ranges from 90.2 to 98.0%. The collaborative disposal of primary ore and multisource solid waste has been achieved through two process paths: reducing smelting and reducing sulfurization smelting, which provide reference for the collaborative smelting of multisource secondary resources.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.028
Threshold uncertainty score0.689

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.239
Teacher spread0.227 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations5
Published2023
Admission routes1
Has abstractyes

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