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Record W4387937498 · doi:10.1002/batt.202300367

Preconditioning Operation of Membraneless Vanadium Micro Redox Flow Batteries

2023· article· en· W4387937498 on OpenAlexaff
Beatriz Oraá‐Poblete, Daniel Pérez-Antolín, Ange A. Maurice, Jesús Palma, Erik Kjeang, Alberto E. Quintero

Bibliographic record

VenueBatteries & Supercaps · 2023
Typearticle
Languageen
FieldEngineering
TopicAdvanced battery technologies research
Canadian institutionsSimon Fraser University
FundersComunidad de Madrid
KeywordsFlow batteryElectrolyteVolumetric flow rateVanadiumMaterials scienceInternal resistanceRedoxDepth of dischargePower densityChemistryAnalytical Chemistry (journal)ElectrodeBattery (electricity)Power (physics)ChromatographyMechanicsThermodynamics

Abstract

fetched live from OpenAlex

Abstract Development of a Membraneless Vanadium Micro Redox Flow Battery (MVMRFB) with an automated closed‐loop control, using micro actuators and micro sensors, is presented for the first‐time during electrolyte preconditioning operation in recirculation mode. The progress of preconditioning is tracked with UV‐vis spectroscopy by 3D printed micro flow cuvettes. Influence of flow rate, reactor internal resistance, and presence of side reactions in the preconditioning process are studied. Optimal flow rate ratio between negative and positive electrolytes is determined and significant performance improvements achieved by operating at lower flow rates are obtained. Influence of reactor internal resistance, which is directly related with the maximum power density, is evaluated demonstrating that operating at a high‐power density can be a source of inefficiency due to the presence of side reactions. Finally, presence of side reactions is evaluated through a dual measurement of electrolytes concentrations in both negative and positive side, and it is demonstrated to be a cause for charge imbalance between the two half‐cells. This work lays a solid foundation for the successful implementation of a charge‐discharge cycle in MVMRFBs operating in recirculation mode.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.045
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.015
GPT teacher head0.245
Teacher spread0.230 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations4
Published2023
Admission routes1
Has abstractyes

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