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Fluctuation stabilization of the <i>Fddd</i> network phase in diblock, triblock, and starblock copolymer melts

2023· article· en· W4388085440 on OpenAlexafffund
M. W. Matsen, T. M. Beardsley, James D. Willis

Bibliographic record

VenuePhysical Review Materials · 2023
Typearticle
Languageen
FieldMaterials Science
TopicBlock Copolymer Self-Assembly
Canadian institutionsUniversity of Waterloo
FundersNatural Sciences and Engineering Research Council of CanadaAlliance de recherche numérique du Canada
KeywordsOrthorhombic crystal systemCopolymerImaging phantomCondensed matter physicsMaterials sciencePhase (matter)Mean field theoryPhysicsThermodynamicsQuantum mechanicsNuclear magnetic resonanceOptics

Abstract

fetched live from OpenAlex

The latest complex network phase to be discovered in diblock copolymer melts is the orthorhombic $F\phantom{\rule{0}{0ex}}d\phantom{\rule{0}{0ex}}d\phantom{\rule{0}{0ex}}d$ phase. Mean-field theory predicts it to be stable, but only at weak segregations where ordered phases are typically destroyed by thermal fluctuations. Indeed, Landau-Brazovskii theory confirmed this expectation, raising the question of how $F\phantom{\rule{0}{0ex}}d\phantom{\rule{0}{0ex}}d\phantom{\rule{0}{0ex}}d$ survives in experiments. However, this problem was recently resolved by accurate field-theoretic simulations, which found that $F\phantom{\rule{0}{0ex}}d\phantom{\rule{0}{0ex}}d\phantom{\rule{0}{0ex}}d$ is simply more resilient to fluctuations than other ordered phases. Here, the authors find that this is also true for the family of (AB)${}_{M}$ starblock copolymer architectures. This resilience may very well extend to numerous other architectures, and thus it would be prudent to keep our eyes open for $F\phantom{\rule{0}{0ex}}d\phantom{\rule{0}{0ex}}d\phantom{\rule{0}{0ex}}d$.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.005
Threshold uncertainty score0.737

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.016
GPT teacher head0.310
Teacher spread0.295 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations11
Published2023
Admission routes2
Has abstractyes

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