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Facilitating the additive manufacture of high-performance polymers through polymer blending: A review

2023· review· en· W4388441758 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

fundA Canadian funder is recorded on the work.
no affNo Canadian affiliation: this work is invisible to an affiliation-only frame.
No Canadian affiliation. An affiliation-only frame, the usual design, would never have seen this work. It is one of the works that make the case for inverting the frame.

Bibliographic record

VenueEuropean Polymer Journal · 2023
Typereview
Languageen
FieldEngineering
TopicAdditive Manufacturing and 3D Printing Technologies
Canadian institutionsnot available
FundersCanada Excellence Research Chairs, Government of CanadaCommonwealth Scientific and Industrial Research Organisation
KeywordsMaterials sciencePolymer3D printingPeekComposite materialExtrusionUltimate tensile strengthPolyetherimideHeat deflection temperatureCrystallizationIzod impact strength testChemical engineering

Abstract

fetched live from OpenAlex

Fused Filament Fabrication (FFF, a.k.a. fused deposition modeling, FDM) is presently the most widespread material extrusion (MEX) additive manufacturing technique owing to its flexibility and robustness. Nonetheless, it remains underutilized in load-bearing applications, as often seen in aerospace, automotive and biomedical industries. This is largely due to the processing challenges associated with high performance polymers (HPPs) like poly-ether-ether-ketone (PEEK) or polyetherimide (PEI). Compared with commercial-grade plastics such as polylactic acid (PLA), parts produced with HPPs have outstanding mechanical properties and thermal stability. However, HPPs have bulkier chemical structures and stronger intermolecular forces than common FFF feedstock materials, and this results in much higher printing temperatures and greater melt viscosities. The demanding processing requirements of HPPs have thus impaired their adoption within FFF. Polymer blending, which consists in properly mixing HPPs with other thermoplastics, makes it possible to alleviate these printing issues, while also providing additional advantages such as improved tensile strength and reduced friction. Further to this, manipulating the crystallisation processes of HPPs mitigates distortion or warping upon printing. This review explores some emerging trends in the field of HPP blends and how they address the challenges of excessive melt viscosity, polymer crystallization, moisture uptake, and part shrinkage in 3D printing. Also, the various structural/mechanical/chemical enhancements that are afforded to FFF parts through HPP blending are critically analysed based on recent examples from the literature. Such insights will not only aid researchers in this field, but also facilitate the development of novel, 3D printable HPP blends.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Research integrity
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Other design · Consensus signal: none
GenreCandidate signal: Review · Consensus signal: Review
Teacher disagreement score0.972
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0020.001
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0020.000
Research integrity0.0000.003
Insufficient payload (model declined to judge)0.0000.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.042
GPT teacher head0.278
Teacher spread0.236 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it