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Record W4388485018 · doi:10.1021/acsestwater.3c00440

Nutrient Impacts on Biogenic Chemical Flux in an End Pit Lake Reclamation Scenario

2023· article· en· W4388485018 on OpenAlexafffund
Najmeh Samadi, Petr Kuznetsov, Alsu Kuznetsova, Julia M. Foght, Ania C. Ulrich, Tariq Siddique

Bibliographic record

VenueACS ES&T Water · 2023
Typearticle
Languageen
FieldEngineering
TopicHydrocarbon exploration and reservoir analysis
Canadian institutionsUniversity of Alberta
FundersNatural Sciences and Engineering Research Council of CanadaSyncrude
KeywordsMethanogenesisEnvironmental chemistryNutrientFlux (metallurgy)ChemistryDissolutionTailingsBiogeochemical cycleMethane

Abstract

fetched live from OpenAlex

Ebullition of biogenic gases, primarily methane (CH 4 ), might affect the trajectory of end pit lake (EPL) reclamation. We investigated the influence of nutrients (N with or without P) on methanogenesis and the resulting chemical flux from underlying fluid fine tailings (FFT) to cap water. Anaerobic 10 L columns were filled with FFT amended with a mixture of hydrocarbons ( n -alkanes, iso -alkanes, and monoaromatics from C 6 –C 10; HC columns) and capped with process water. Some amended FFT were further amended with N (HCN columns) or N and P (HCNP columns). A microbial community dominated by Desulfobacterota and Desulfotomaculales plus acetoclastic and hydrogenotrophic methanogens depleted hydrocarbons at different rates concomitant with CH 4 production in the order HCN > HC > HCPN, indicating stimulation of methanogenesis by N and inhibition by P amendments. Microbial processes transformed FFT minerals (Fe III to Fe II minerals and dissolution of carbonates), mobilized ions, and trace elements (Ca 2+, Mg 2+, K +, HCO 3 –, Sr, and Ba) in FFT porewater and densified FFT and induced chemical flux to cap water. Other dissolved trace elements (As, Sb, and Mo) decreased in porewater and cap water during methanogenesis. The results provide novel information about nutrients’ effect on methanogenesis and associated chemical flux to inform predictions about sustainable management of EPL.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.043
Threshold uncertainty score0.085

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0010.000
Scholarly communication0.0010.001
Open science0.0000.001
Research integrity0.0010.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.017
GPT teacher head0.236
Teacher spread0.219 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations3
Published2023
Admission routes2
Has abstractyes

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