MétaCan
Menu
← all works

Improving Electrocatalytic Oxygen Evolution through Local Field Distortion in Mg/Fe Dual‐site Catalysts

2023· article· en· 100 citations· W4388531183 on OpenAlex· 10.1002/anie.202314303

Why is this work in the frame?

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

Canadian affiliationAn author listed a Canadian institution. This is the only route the usual frame has.

Full frame distilled prediction

Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

Candidate categories
Meta-epidemiology (narrow)
Consensus categories
none
Domain
Candidate signal: noneConsensus signal: none
Study design
Candidate signal: Bench or experimentalConsensus signal: Bench or experimental
Genre
Candidate signal: EmpiricalConsensus signal: Empirical
Teacher disagreement score
0.076
Threshold uncertainty score
1.000
Validation status
machine_predicted_unvalidated · codex-gemma-dda1882f352a

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Opus teacher head0.009
GPT teacher head0.236
Teacher spread
0.227 · how far apart the two teachers sit on this one work
Validation status
score_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Abstract

Abstract Transition metal single atom electrocatalysts (SACs) with metal‐nitrogen‐carbon (M−N−C) configuration show great potential in oxygen evolution reaction (OER), whereby the spin‐dependent electrons must be allowed to transfer along reactants (OH − /H 2 O, singlet spin state) and products (O 2 , triplet spin state). Therefore, it is imperative to modulate the spin configuration in M−N−C to enhance the spin‐sensitive OER energetics, which however remains a significant challenge. Herein, we report a local field distortion induced intermediate to low spin transition by introducing a main‐group element (Mg) into the Fe−N−C architecture, and decode the underlying origin of the enhanced OER activity. We unveil that, the large ionic radii mismatch between Mg 2+ and Fe 2+ can cause a FeN 4 in‐plane square local field deformation, which triggers a favorable spin transition of Fe 2+ from intermediate (d xy 2 d xz 2 d yz 1 d z2 1 , 2.96 μ B ) to low spin (d xy 2 d xz 2 d yz 2 , 0.95 μ B ), and consequently regulate the thermodyna‐mics of the elementary step with desired Gibbs free energies. The as‐obtained Mg/Fe dual‐site catalyst demonstrates a superior OER activity with an overpotential of 224 mV at 10 mA cm −2 and an electrolysis voltage of only 1.542 V at 10 mA cm −2 in the overall water splitting, which outperforms those of the state‐of‐the‐art transition metal SACs.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

The record

Venue
Angewandte Chemie International Edition
Topic
Electrocatalysts for Energy Conversion
Field
Energy
Canadian institutions
Canadian Light Source (Canada)University of Saskatchewan
Funders
National Natural Science Foundation of China
Keywords
Oxygen evolutionSpin statesOverpotentialIonic bondingChemistryTransition metalSpin transitionCatalysisSinglet stateSpin crossoverChemical physicsCrystallographyMaterials scienceAtomic physicsIonInorganic chemistryPhysical chemistryPhysicsExcited stateElectrodeElectrochemistry
Has abstract in OpenAlex
yes