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Record W4388572559 · doi:10.1002/vzj2.20292

Quantitative analysis of diurnal CO <sub>2</sub> flux variations above an alkaline playa

2023· article· en· W4388572559 on OpenAlexafffund
Anne‐Martine Doucet, Frances Jones, Katherine E. Raymond, Gregory M. Dipple, Bethany Ladd, K. Ulrich Mayer

Bibliographic record

VenueVadose Zone Journal · 2023
Typearticle
Languageen
FieldEnvironmental Science
TopicCO2 Sequestration and Geologic Interactions
Canadian institutionsSaskatoon Medical ImagingArcadis (Canada)University of British Columbia
FundersNatural Sciences and Engineering Research Council of CanadaNatural Resources CanadaCanada Foundation for Innovation
KeywordsAtmosphere (unit)Carbon dioxideCarbonateFlux (metallurgy)Atmospheric sciencesDaytimeChemistryLimitingBicarbonateDiurnal temperature variationEnvironmental scienceEnvironmental chemistryMineralogyGeologyMeteorology

Abstract

fetched live from OpenAlex

Abstract The alkaline playas at Atlin, BC, provide a unique opportunity for studying the carbonate–bicarbonate system and carbonate mineral stability at the Earth's surface. In this study, dynamic closed chambers (DCCs) and pore‐gas sampling were used to directly quantify carbon dioxide (CO 2 ) emission rates and characterize processes governing the CO 2 exchange across the playa‐atmosphere interface. Data were collected at the Atlin site continuously over 27 days in 2020 and 14 days in 2021. Results indicate minimal net exchange of CO 2 across the playa‐atmosphere interface during the monitoring periods, with average fluxes over the two periods of −0.03 and 0.09 µmol m −2 s −1 in 2020 and 2021, respectively. However, distinct diurnal oscillations of CO 2 fluxes were measured with average daytime fluxes of 0.15 ± 0.34 µmol m −2 s −1 (2020) and 0.15 ± 0.19 µmol m −2 s −1 (2021) and nighttime fluxes of −0.24 ± 0.31 µmol m −2 s −1 (2020) and 0.04 ± 0.18 µmol m −2 s −1 (2021). These observations, supported by reactive transport modeling, indicate that CO 2 exchange is predominantly governed by changes in CO 2 solubility in alkaline porewater related to diurnal temperature fluctuations and variations in CO 2 concentrations in ambient air above the ground surface. Even though CO 2 concentrations exceed 8000 ppmv at 1‐m depth, CO 2 emissions to the atmosphere were found to be minimal, likely due to high moisture contents, low connectivity, and tortuosity, limiting upward CO 2 migration. These findings provide insights into CO 2 flux dynamics in alkaline arid regions and show promise for the application of the DCC method for monitoring ex situ carbon mineralization at sites with enhanced mineral weathering.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesInsufficient payload (model declined to judge)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.731
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.002
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0080.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.029
GPT teacher head0.314
Teacher spread0.285 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; both teacher heads agree on what is shown here.

Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2023
Admission routes2
Has abstractyes

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