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Record W4388938333 · doi:10.1002/pen.26568

Influence of polymer solution composition on the microstructure and thermal and mechanical characteristics of polycaprolactone films

2023· article· en· W4388938333 on OpenAlexafffund
Hassan Sawalha, Theo G. M. van de Ven

Bibliographic record

VenuePolymer Engineering and Science · 2023
Typearticle
Languageen
FieldMaterials Science
Topicbiodegradable polymer synthesis and properties
Canadian institutionsMcGill UniversityMcGill University Health Centre
FundersFonds de recherche du Québec – Nature et technologiesFonds de Recherche du Québec - SantéCentre québécois sur les matériaux fonctionnelsFonds de Recherche du Québec-Société et CultureMcGill University
KeywordsMaterials sciencePolycaprolactoneMicrostructureCrystallinityComposite materialPolymerCastingUltimate tensile strengthHexadecaneChemical engineeringOrganic chemistryChemistry

Abstract

fetched live from OpenAlex

Abstract This study investigates the effects of addition of oils and alkanes to the polymer solution on the properties of polycaprolactone (PCL) films. The films were prepared by casting films onto a mold and evaporation in air. Films made without oils showed a dense microstructure. Most of the oils generated porous films, except for cyclohexane and castor oil. The neat PCL and cyclohexane films were stronger than other films, with a tensile strength of about ~11.5 MPa, followed by terpenes (~6.5 MPa) and the weakest films were obtained with hexadecane (~3.5 MPa). The elastic modulus was highest with limonene (~350 MPa), followed by cyclohexane (~150 MPa), and the lowest modulus (~65 MPa) was obtained with castor oil and hexadecane. All films showed high elongation at break (>400%). The degree of crystallinity was the highest with terpenes, whereas the lowest crystallinity was obtained with hexadecane. No significant effect of the oils on the thermal transition temperatures of the films could be observed. In summary, the microstructure and mechanical properties of the PCL films could be effectively fine‐tuned for various applications through the addition of oils and alkanes to the polymer solution. Highlights Oils and alkanes were added to polycaprolactone (PCL) casting solution. PCL films were prepared by casting films onto a mold and evaporation in air. Oils affected the microstructure and mechanical properties of the films. Addition of oils provides a flexible tool to tailor the film properties. PCL films with varying properties could be fabricated for different fields.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.033
Threshold uncertainty score0.287

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.200
Teacher spread0.189 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations4
Published2023
Admission routes2
Has abstractyes

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