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Record W4389042127 · doi:10.1021/acs.iecr.3c02592

Atomistic Analysis of the Microbial Influence on the Adsorption Characteristic of Sulfur, Hydrogen, and SO<sub>4</sub>on Iron Surfaces

2023· article· en· W4389042127 on OpenAlexafffund
Mohammad Asif, Faisal Khan, Kelly Hawboldt

Bibliographic record

VenueIndustrial & Engineering Chemistry Research · 2023
Typearticle
Languageen
FieldMaterials Science
TopicCorrosion Behavior and Inhibition
Canadian institutionsMemorial University of Newfoundland
FundersCanada Research ChairsGenome Canada
KeywordsSulfurAdsorptionCorrosionHydrogenElectric fieldMetalChemistryInorganic chemistryElectron transferDensity functional theoryMaterials scienceChemical physicsChemical engineeringMetallurgyPhysical chemistryComputational chemistryOrganic chemistry

Abstract

fetched live from OpenAlex

The corrosion of metals is enhanced by the presence of microbes on the surface; however, the mechanisms governing this impact are poorly understood. This study used a molecular modeling approach to understand microbial activity on a metal surface. As microbes can remove protons from the biofilm or consume electrons from the iron surface, this electron transfer activity is modeled in density functional theory as an external electric field. Three corrosion-causing components, (i) sulfur, (ii) hydrogen, and (iii) SO 4, are studied over iron surfaces. It is observed that the adsorption energy of SO 4, sulfur, and hydrogen on Fe (100), Fe (110), and Fe (310) surfaces increased with the applied electric field, irrespective of the direction (positive/negative) of the electric field. The Fe (110) surface is more stable than the Fe (100) and Fe (310) surfaces for the adsorption of sulfur and SO 4, even at higher electric fields and concentrations of the components. This confirms the common understanding that Fe (110) is a higher corrosion resistive compared to Fe (100) and Fe (310). Further investigation is performed using population analysis, electronic density of states, and density difference. This analysis confirms Fe (110) microbial corrosion resistance characteristics.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.012
Threshold uncertainty score0.023

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0000.000
Science and technology studies0.0010.001
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0010.000
Insufficient payload (model declined to judge)0.0030.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.054
GPT teacher head0.291
Teacher spread0.237 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations3
Published2023
Admission routes2
Has abstractyes

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