MétaCan
Menu
Back to cohort
Record W4389076650 · doi:10.1021/acs.chemmater.3c01675

Porous Semiconducting K–Sn–Mo–S Aerogel: Synthesis, Local Structure, and Ion-Exchange Properties

2023· article· en· W4389076650 on OpenAlexafffund
Alicia Blanton, Taohedul Islam, Subrata Chandra Roy, Ahmet Çelik, Jing Nie, David R. Baker, Dien Li, K. Taylor-Pashow, Xianchun Zhu, Avijit Pramanik, Ruhul Amin, Renfei Feng, Roman Chernikov, Saiful M. Islam

Bibliographic record

VenueChemistry of Materials · 2023
Typearticle
Languageen
FieldChemistry
TopicRadioactive element chemistry and processing
Canadian institutionsCanadian Light Source (Canada)
FundersSavannah River National LaboratoryNational Institute on Minority Health and Health DisparitiesDivision of ChemistryCanadian Light SourceNatural Sciences and Engineering Research Council of CanadaJackson State UniversityOffice of ScienceBritish Society for Research on AgeingUniversity of ChicagoNational Science FoundationCanadian Institutes of Health ResearchU.S. Department of EducationArgonne National LaboratoryDivision of Electrical, Communications and Cyber SystemsU.S. Department of EnergyNational Institutes of Health
KeywordsAmorphous solidExtended X-ray absorption fine structureIon exchangeChemistryAerogelAbsorption (acoustics)TinCovalent bondSorptionCoordination numberIonInorganic chemistryMaterials scienceCrystallographyPhysical chemistryNanotechnologyAbsorption spectroscopyAdsorptionOrganic chemistry

Abstract

fetched live from OpenAlex

Chalcogenide-based aerogels are emerging porous semiconducting nanomaterials that appeal to applications in clean energy and the environment. Here, we report a novel gel, potassium–tin–molybdenum–sulfides (KTMS), that integrates the electrostatically bound K + ions in the covalent network of Sn–Mo–S. Its gelation requires a concurrent reduction of Mo 6+ → Mo 4+/5+ and the oxidation of S 2– → S n – ( n ≈ 1) and Sn 2+ → Sn 4+ . KTMS is an amorphous semiconductor showing quantum confinement effects on band gap energies, 2.1 → 1.4 → 0.9 eV for its wet- → aero- → xerogels. Synchrotron X-ray pair distribution function (PDF) and extended X-ray absorption fine structure (EXAFS) revealed a complex local structure of KTMS consisting of molecular Mo 2 (S 2 ) 6 and Mo 3 S(S 2 ) 6 clusters. In addition, the Sn–S coordination is related to crystalline Na 4 Sn 3 S 8 and SnS 2 . KTMS also demonstrated the removal of the radionuclides of Cs +, Sr 2+, and UO 2 2+ from ppm to ppb levels with distribution constants ( K d ) up to ≥10 4 mL/g. Notably, despite the lack of atomic periodicity in the amorphous KTMS, the K + ion is ion-exchangeable with chemically diverse Sr 2+, Cs +, and UO 2 2+ in aqueous solutions; especially the ion-exchange properties of Sr 2+ and UO 2 2+ ≡(O═U═O) 2+ is not known to any chalcogels known to date. The sequestration of Cs + and Sr 2+ was achieved by the exchange of K + in the amorphous KTMS, and the removal of [O═U 6+ ═O] 2+ synergistically involves surface sorption via ─S ···· U 6+ ═O 2 2+ covalent interactions and ion-exchange via the hard–soft Lewis acid–base paradigm. Overall, cooperative roles played by the diverse bonding motifs, surface-exposed Lewis basic frameworks, and polarizability of the (poly)sulfides make it an exceptional adsorbent for chemically diverse radioactive species. This finding will guide the design of superior sorbents for chemically distinct metal ion separation.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.006
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0030.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.027
GPT teacher head0.238
Teacher spread0.211 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations10
Published2023
Admission routes2
Has abstractyes

Explore more

Same venueChemistry of MaterialsSame topicRadioactive element chemistry and processingFrench-language works237,207