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Record W4389584974 · doi:10.17118/11143/21066

Functionalized graphene nanosheets as filtration membranes for theremoval of Cd2+ from wastewater

2023· article· en· W4389584974 on OpenAlexaff
Akram Khalajiolyaie, Cuiying Jian

Bibliographic record

Venuenot available
Typearticle
Languageen
FieldChemistry
TopicNanomaterials for catalytic reactions
Canadian institutionsYork University
Fundersnot available
KeywordsFiltration (mathematics)MembraneWastewaterGrapheneChemical engineeringMaterials scienceNanotechnologyWaste managementPulp and paper industryChemistryEnvironmental scienceEnvironmental engineeringEngineeringMathematics

Abstract

fetched live from OpenAlex

Toxic metals such as Pb, Cu, Cd, Zn, Ag, and Hg can be seen in industrial wastewater. The existence of these heavy metals in environment can cause liver and kidney disease, and thus is extremely harmful. Filtration-based membranes, such as reverse osmosis and nanofiltration membranes, can help to remove heavy metals from contaminated water by physical separation. The membrane acts as a barrier that allows only water molecules to pass through, while blocking pollutants, e.g., heavy metal ions. The process can effectively reduce the concentration of heavy metals in water, making it safer for consumption and other uses. In this study, the performance of nonporous graphene (NPG), which is functionalized by hydrogen (NPG-H) and hydroxyl (NPG-OH) as a nanostructure membrane, has been investigated by molecular dynamics techniques. These membranes had two different pore sizes, for which the radius is 5 and 10 , respectively, leading to 4 different types of membranes. An external pressure was applied to the system to mimic pressure-driven filtrations. It was found that with a small pore (5 ), both NPG-H and NPG-OH totally rejected Cd 2+ and Cl -1 , while with a large pore (10 ), Cd 2+ gradually passed through NPG-H and NPG-OH membranes. In terms of water molecules filtered, membranes with large pores have a larger permeability compared to those with small pores. For the effects of functional groups, compared to NPG-OH, NPG-H can allow more water molecules to permeate the pore, regardless of pore sizes. On the other hand, the rejection rates of functional groups for Cd 2+ and Cl -1 show dependences on pore sizes. The underlying mechanisms for these observations will be explored. The results obtained shed lights on the effects of pore sizes and functional groups on water permeability and Cd 2+ rejection rate for graphene-based filtration membranes.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0010.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.022
GPT teacher head0.256
Teacher spread0.234 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2023
Admission routes1
Has abstractyes

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