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Record W4389686418 · doi:10.1021/acssuschemeng.3c06351

Improvement in the Thermomechanical Properties and Adhesion of Wood Fibers to the Polyamide 6 Matrix by Sequential Ball Milling Technique

2023· article· en· W4389686418 on OpenAlexafffund
Adel Jalaee, E. Johan Foster

Bibliographic record

VenueACS Sustainable Chemistry & Engineering · 2023
Typearticle
Languageen
FieldMaterials Science
TopicNatural Fiber Reinforced Composites
Canadian institutionsUniversity of British Columbia
FundersNatural Sciences and Engineering Research Council of CanadaCanada Foundation for Innovation
KeywordsMaterials scienceComposite materialAbsorption of waterBall millCelluloseDynamic mechanical analysisPolyamidePulp (tooth)Environmentally friendlyComposite numberPolymerChemical engineering

Abstract

fetched live from OpenAlex

The engineering thermoplastics industry has largely limited the use of natural fiber reinforcements due to their susceptibility to low-onset thermal degradation and water absorption. Therefore, in order to utilize these economically viable and environmentally friendly materials effectively through common composite fabrication methods such as hot pressing, safeguarding them from thermal degradation becomes essential. This work presents a viable industrially technique called sequential ball milling for processing unbleached softwood kraft pulp fibers (PF) with an engineering thermoplastics polyamide 6 (PA6) with high melting temperatures (>220 °C). An additional eco-friendly modification step that employs ball milling and cellulose nanocrystal (CNC) has been implemented in this study to enhance the mechanical properties of the composites. Special attention is given to fine-tuning key variables, such as milling duration and PF particle size, to produce optimal composites. Leveraging the ability of sequential ball milling to evenly distribute pulp fibers into PA6, a 160% increase in Young's modulus was achieved with the incorporation of 30 wt % PF. Importantly, the introduction of a 5 wt % CNC modifying agent elevated Young's modulus to 4.3 GPa, marking a 187% improvement over unmodified PA6. Diverse techniques, including rheological analyses, thermomechanical evaluations, morphological examinations, and assessments of moisture absorption, were utilized to validate the efficiency of the suggested processing approach and the modification phase.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.003
Threshold uncertainty score0.405

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.212
Teacher spread0.204 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations11
Published2023
Admission routes2
Has abstractyes

Explore more

Same venueACS Sustainable Chemistry & EngineeringSame topicNatural Fiber Reinforced CompositesFrench-language works237,207