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Record W4389883445 · doi:10.1021/acsami.3c12381

Albumin Protein Impact on Early-Stage <i>In Vitro</i> Biodegradation of Magnesium Alloy (WE43)

2023· article· en· W4389883445 on OpenAlexafffund
Amin Imani, Ehsan Rahimi, Maria Lekka, Francesco Andreatta, Michele Magnan, Yaiza González‐García, J.M.C. Mol, R.K. Singh Raman, L. Fedrizzi, Edouard Asselin

Bibliographic record

VenueACS Applied Materials & Interfaces · 2023
Typearticle
Languageen
FieldMaterials Science
TopicMagnesium Alloys: Properties and Applications
Canadian institutionsUniversity of British Columbia
FundersTechnische Universiteit DelftDelft Research CentresNatural Sciences and Engineering Research Council of CanadaUniversità degli Studi di UdineUniversity of British ColumbiaMonash University
KeywordsBiocompatibilityMaterials scienceBovine serum albuminBiodegradationAlloyCorrosionElectrochemistryNuclear chemistryChemical engineeringMetallurgyChromatographyElectrodeChemistryOrganic chemistry

Abstract

fetched live from OpenAlex

High Resolution Image Download MS PowerPoint Slide Mg and its alloys are promising biodegradable materials for orthopedic implants and cardiovascular stents. The first interactions of protein molecules with Mg alloy surfaces have a substantial impact on their biocompatibility and biodegradation. We investigate the early-stage electrochemical, chemical, morphological, and electrical surface potential changes of alloy WE43 in either 154 mM NaCl or Hanks’ simulated physiological solutions in the absence or presence of bovine serum albumin (BSA) protein. WE43 had the lowest electrochemical current noise (ECN) fluctuations, the highest noise resistance ( Z n = 1774 Ω·cm 2 ), and the highest total impedance (| Z | = 332 Ω·cm 2 ) when immersed for 30 min in Hanks’ solution. The highest ECN, lowest Z n (1430 Ω·cm 2 ), and |Z| (49 Ω·cm 2 ) were observed in the NaCl solution. In the solutions containing BSA, a unique dual-mode biodegradation was observed. Adding BSA to a NaCl solution increased | Z | from 49 to 97 Ω·cm 2 and decreased the ECN signal of the alloy, i.e., the BSA inhibited corrosion. On the other hand, the presence of BSA in Hanks’ solution increased the rate of biodegradation by decreasing both Z n and | Z | while increasing ECN. Finally, using scanning Kelvin probe force microscopy (SKPFM), we observed an adsorbed nanolayer of BSA with aggregated and fibrillar morphology only in Hanks’ solution, where the electrical surface potential was 52 mV lower than that of the Mg oxide layer.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesInsufficient payload (model declined to judge)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.002

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.018
GPT teacher head0.258
Teacher spread0.240 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; both teacher heads agree on what is shown here.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations24
Published2023
Admission routes2
Has abstractyes

Explore more

Same venueACS Applied Materials & InterfacesSame topicMagnesium Alloys: Properties and ApplicationsFrench-language works237,207