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Record W4390056837 · doi:10.1002/cjce.25165

Machine learning techniques for the prediction of polymerization kinetics and polymer properties

2023· article· en· W4390056837 on OpenAlexvenueno aff
Niyi B. Ishola, Timothy F. L. McKenna

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2023
Typearticle
Languageen
FieldEngineering
TopicFuel Cells and Related Materials
Canadian institutionsnot available
FundersPetroleum Technology Development Fund
KeywordsAdaptive neuro fuzzy inference systemIsopentanePolymerizationExtreme learning machineMelt flow indexBiological systemCoefficient of determinationSensitivity (control systems)Mean squared errorPolymerMaterials scienceComputer scienceMathematicsMachine learningChemistryArtificial intelligenceStatisticsFuzzy logicEngineeringOrganic chemistryCatalysisComposite materialArtificial neural networkFuzzy control system

Abstract

fetched live from OpenAlex

Abstract In the current study, the ability of two data‐driven machine learning tools, the extreme learning machine (ELM) and the adaptive neuro‐fuzzy inference system (ANFIS), to predict the polymerization rate and melt flow index of linear low‐density polyethylene produced in a gas phase process was investigated. The level of interaction between the input variables (ethylene, 1‐butene, isopentane pressures, and reaction temperature) on the outputs (melt flow index and activity) was also examined. It was found that both outputs are impacted by the presence of isopentane as an induced condensing agent. Various statistical indicators, including the coefficient of correlation ( R 2 ) and root mean square error (RMSE), were used to quantitatively evaluate both developed models. The ANFIS model outperformed the developed ELM model in terms of predicting the MFI and the catalyst activity. A sensitivity analysis of the ANFIS and ELM models showed that all the input variables under investigation had a sizable impact on the responses and none of them could have been discarded. The present study showed that machine learning tools could be employed to adequately develop empirical models to predict polymerization kinetics as well as the final polymer properties.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.004
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: Simulation or modeling
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.003
Threshold uncertainty score0.007

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0010.004
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0010.000
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.163
Teacher spread0.155 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations10
Published2023
Admission routes1
Has abstractyes

Explore more

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