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Record W4390229926 · doi:10.26434/chemrxiv-2023-c1c33

Improving the Conductance Blockage Model of Cylindrical Nanopores – from 2D to Thick Membranes

2023· preprint· en· W4390229926 on OpenAlexafffund
Martin Charron, Zachary Roelen, Vincent Tabard‐Cossa

Bibliographic record

VenueChemRxiv · 2023
Typepreprint
Languageen
FieldEngineering
TopicNanopore and Nanochannel Transport Studies
Canadian institutionsUniversity of Ottawa
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsNanoporeConductanceMembraneMaterials scienceMoleculeNanotechnologyMechanicsChemical physicsBiological systemChemistryPhysicsCondensed matter physics

Abstract

fetched live from OpenAlex

The ionic current blockage from a nanopore sensor is a fundamental metric for characterizing its dimensions and for sizing and identifying molecules translocating through. Yet, models for precisely predicting the conductance of a nanopore in both an open and a blocked state are lacking, which leads to significant errors in the determination of the expected blockage depth from a given translocating molecule and of the pore diameter and length. Here, using oblate spheroidal coordinates as a framework to study the conductance of a nanopore, we demonstrate that the widely used Kowalczyk et al. model significantly overestimates the contribution from the access region in the presence of a cylindrical obstruction. We present a highly precise analytical model for the blocked conductance of 2D nanopores and extend it to cylindrical pores of varying membrane thicknesses. Using finite element simulations, our results show that errors in the calculation of the conductance blockage are maximal for pores with aspect ratios of d/L≈5, but are minimal for both d/L≫1 and d/L≪1. The model presented is especially precise for ultra-thin membranes, with prediction errors below 3% for all pore sizes tested with a membrane thickness of 0.3 nm. By improving on the conductance model of the nanopore system, more accurate estimates of the expected blockage depth from a translocating molecule and of pore dimensions can be obtained, with great practical value for many biosensing applications.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: Simulation or modeling
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.007
Threshold uncertainty score0.014

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0000.000
Science and technology studies0.0000.001
Scholarly communication0.0010.001
Open science0.0010.001
Research integrity0.0020.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.042
GPT teacher head0.237
Teacher spread0.195 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2023
Admission routes2
Has abstractyes

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