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Elemental dynamics and interactions in a carbonate-buffered, sulfatic and ferruginous lake

2023· preprint· en· W4390271512 on OpenAlexaff
Daniel A. Petrash, Christophe Thomazo, Astolfo Valero, James J. Valdés, Karelys Umbría-Salinas, Travis B. Meador, Vladislav Chrastný, Kurt O. Konhauser

Bibliographic record

Venuenot available
Typepreprint
Languageen
FieldEarth and Planetary Sciences
TopicGeochemistry and Elemental Analysis
Canadian institutionsUniversity of Alberta
FundersUniversité de Bretagne Occidentale
KeywordsAnoxic watersCarbonateWater columnBiogeochemical cycleSulfateEnvironmental chemistryRedoxPyriteGeologyDissolutionSulfurTrace metalChemistryGeochemistryInorganic chemistryMetalOceanography

Abstract

fetched live from OpenAlex

Lake Medard is a recently established post-mining lake in the northwest of Czech Republic that displays significant concentrations of dissolved sulfate (dSO42-) and ferrous iron (Fe2+) in its density and redox stratified bottom water column. Siderite-buffered anoxic sediments, also rich in iron(III)-oxyhydroxides, underlie that water column characterized by limited labile organic substrates. This composition sustain a transitional redox state between nitrogenous/ferruginous and euxinic conditions. Our study focuses on the Lake Medard bottom water column elemental concentration profiles, sulfate-sulfur and -oxygen isotope compositions, bioactive ion concentrations, and planktonic microbiome data, combined with mineralogical and isotopic analyses of the upper anoxic sediments. This integrative approach reveals that the internal biogeochemical iron cycling is interlinked with that of nitrogen, sulfur and other redox sensitive metals. Minor seasonal oscillations in the monimolimnion redox potential impact mineral dissolution/(re)precipitation reactions, causing shifts in metal partitioning within anoxic sediments. Carbonate-buffered reactions appear to respond to a subsurface CO2 flux thereby influencing monimolimnial alkalinity and dissolved inorganic carbon concentrations. These hydrochemical modifications shift the sedimentary redox signals, occasionally favoring carbonate over oxyhydroxide metal-binding processes. Our findings address the fate of newly formed sedimentary oxyhydroxides in a transitional redox-stratified water column featuring ferruginous conditions without quantitative sulfate depletion to provide insights on interlinked biogeochemical processes within a concise framework

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.025
Threshold uncertainty score0.049

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0010.000
Scholarly communication0.0010.000
Open science0.0000.001
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.022
GPT teacher head0.239
Teacher spread0.217 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2023
Admission routes1
Has abstractyes

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