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Record W4390741104 · doi:10.1515/nanoph-2023-0687

Modeling with graded interfaces: Tool for understanding and designing record‐high power and efficiency mid‐infrared quantum cascade lasers

2024· article· en· W4390741104 on OpenAlexaff
Suraj Suri, B. Knipfer, Thomas Grange, Huilong Gao, Jeremy Kirch, L. J. Mawst, Robert A. Marsland, D. Botez

Bibliographic record

VenueNanophotonics · 2024
Typearticle
Languageen
FieldChemistry
TopicSpectroscopy and Laser Applications
Canadian institutionsNexen (Canada)
FundersNaval Air Systems CommandNational Institute of Environmental Health SciencesU.S. NavyUniversity of Wisconsin-Madison
KeywordsCascadeOptoelectronicsNanomaterialsInfraredQuantumLaserMaterials scienceQuantum cascade laserPower (physics)Computer scienceNanotechnologyOpticsPhysicsEngineering

Abstract

fetched live from OpenAlex

Abstract By employing a graded‐interfaces model based on a generalized formalism for interface‐roughness (IFR) scattering that was modified for mid‐infrared emitting quantum cascade lasers (QCLs), we have accurately reproduced the electro‐optical characteristics of published record‐performance 4.9 µm‐ and 8.3 µm‐emitting QCLs. The IFR‐scattering parameters at various interfaces were obtained from measured values and trends found via atom‐probe tomography analysis of one of our 4.6 μm‐emitting QCL structures with variable barrier heights. Those values and trends, when used for designing a graded‐interface, 4.6 μm‐emitting QCL, led to experimental device characteristics in very good agreement with calculated ones. We find that the published record‐high performance values are mainly due to both injection from a prior‐stage low‐energy (active‐region) state directly into the upper‐laser ( ul ) level, thus at low field‐strength values, as well as to strong photon‐induced carrier transport. However, the normalized leakage‐current density J leak / J is found to be quite high: 26–28 % and 23.3 %, respectively, mainly because of IFR‐triggered shunt‐type leakage through high‐energy active‐region states, in the presence of high average electron temperatures in the ul laser level and an energy state adjacent to it: 1060 K and 466 K for 4.9 µm‐ and 8.3 µm‐emitting QCLs, respectively. Then, modeling with graded interfaces becomes a tool for designing devices of performances superior to the best reported to date, thus closing in on fundamental limits. The model is employed to design a graded‐interface 8.1 µm‐emitting QCL with suppressed carrier leakage via conduction‐band engineering, which reaches a maximum front‐facet wall‐plug efficiency value of 22.2 %, significantly higher than the current record (17 %); thus, a value close to the fundamental front‐facet, upper limit (i.e., 25 %) for ∼8 µm‐emitting QCLs.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.713
Threshold uncertainty score0.710

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.023
GPT teacher head0.259
Teacher spread0.236 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations14
Published2024
Admission routes1
Has abstractyes

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