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Record W4391011526 · doi:10.1021/acsapm.3c02531

Surface Modification and Dyeing of Ultrahigh-Molecular-Weight Polyethylene Fabrics Using Diazirine-Based Polymers

2024· article· en· W4391011526 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueACS Applied Polymer Materials · 2024
Typearticle
Languageen
FieldEngineering
TopicAdvanced Sensor and Energy Harvesting Materials
Canadian institutionsUniversity of Victoria
FundersMitacsInnovate BC
KeywordsCovalent bondSurface modificationMaterials sciencePolyethyleneEpoxyPolymerComposite materialPolymer chemistryUltra-high-molecular-weight polyethyleneAdhesionCoatingPolyamineChemical engineeringChemistryOrganic chemistry

Abstract

fetched live from OpenAlex

Ultrahigh-molecular-weight polyethylene (UHMWPE) fibers are valued for their high strength-to-weight ratio and are employed in a wide variety of commercial applications. However, because of its low surface energy, UHMWPE can fail in certain applications such as fiber-reinforced composites. This is due to its poor interfacial adhesion with polar matrices, making it challenging to incorporate into composites or retain polar dyes or colorants. Herein, we describe the use of polyamine primers for coating UHMWPE weaves, covalently bonding the aliphatic chains through C–H insertion, leading to strong covalent interactions between the fabric and polyamines. We further demonstrate that the polyamine-coated UHMWPE surfaces can successfully react with epoxy resin through nucleophilic addition reactions to enable the production of epoxy composites. Furthermore, we show the use of polyamine-coated UHMWPE in secondary functionalization with amine-reactive compounds, such as dyes, through covalent linkages that result in very strong color fastness.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.026
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.014
GPT teacher head0.235
Teacher spread0.221 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it