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Record W4391262708 · doi:10.1038/s41563-024-01797-0

Absence of 3a0 charge density wave order in the infinite-layer nickelate NdNiO2

2024· article· en· W4391262708 on OpenAlexafffund
C. T. Parzyck, Naman Gupta, Y. Wu, V. Anil, Lopa Bhatt, M. Bouliane, Rantong Gong, Benjamin Gregory, Aileen Luo, Ronny Sutarto, Feizhou He, Yi‐De Chuang, Tao Zhou, G. Herranz, Lena F. Kourkoutis, Andrej Singer, Darrell G. Schlom, D. G. Hawthorn, Kyle Shen

Bibliographic record

VenueNature Materials · 2024
Typearticle
Languageen
FieldMaterials Science
TopicMagnetic and transport properties of perovskites and related materials
Canadian institutionsCanadian Light Source (Canada)University of Waterloo
FundersDivision of Materials ResearchNational Science FoundationCanadian Institutes of Health ResearchCornell Center for Materials ResearchOffice of ScienceGeneralitat de CatalunyaMinisterio de Ciencia e InnovaciónKavli Institute at Cornell, Cornell UniversityGordon and Betty Moore FoundationArgonne National LaboratoryU.S. Department of EnergyU.S. Department of DefenseBasic Energy SciencesNatural Sciences and Engineering Research Council of CanadaCanadian Light Source
KeywordsCuprateCondensed matter physicsSuperconductivityCharge density waveSuperlatticeCharge (physics)Order (exchange)ScatteringPhysicsCharge densityPhase (matter)Materials scienceQuantum mechanics

Abstract

fetched live from OpenAlex

Abstract A hallmark of many unconventional superconductors is the presence of many-body interactions that give rise to broken-symmetry states intertwined with superconductivity. Recent resonant soft X-ray scattering experiments report commensurate 3 a 0 charge density wave order in infinite-layer nickelates, which has important implications regarding the universal interplay between charge order and superconductivity in both cuprates and nickelates. Here we present X-ray scattering and spectroscopy measurements on a series of NdNiO 2+ x samples, which reveal that the signatures of charge density wave order are absent in fully reduced, single-phase NdNiO 2 . The 3 a 0 superlattice peak instead originates from a partially reduced impurity phase where excess apical oxygens form ordered rows with three-unit-cell periodicity. The absence of any observable charge density wave order in NdNiO 2 highlights a crucial difference between the phase diagrams of cuprate and nickelate superconductors.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.020
Threshold uncertainty score0.993

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0010.000
Insufficient payload (model declined to judge)0.0080.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.238
Teacher spread0.226 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations58
Published2024
Admission routes2
Has abstractyes

Explore more

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