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Record W4391320928 · doi:10.1002/bte2.20230062

Lithium dendrites in all‐solid‐state batteries: From formation to suppression

2024· article· en· W4391320928 on OpenAlexafffund
Huaihu Sun, Axel Celadon, Sylvain G. Cloutier, Kamal Al‐Haddad, Shuhui Sun, Gaixia Zhang

Bibliographic record

VenueBattery energy · 2024
Typearticle
Languageen
FieldEngineering
TopicAdvanced Battery Materials and Technologies
Canadian institutionsÉcole de Technologie SupérieureInstitut National de la Recherche Scientifique
FundersCentre québécois sur les matériaux fonctionnelsNatural Sciences and Engineering Research Council of CanadaÉcole de technologie supérieureInstitut national de la recherche scientifique
KeywordsSolid-stateLithium (medication)Materials scienceNanotechnologyChemical engineeringEngineering physicsPsychologyPhysicsEngineering

Abstract

fetched live from OpenAlex

Abstract All‐solid‐state lithium (Li) metal batteries combine high power density with robust security, making them one of the strong competitors for the next generation of battery technology. By replacing the flammable and volatile electrolytes commonly found in traditional Li‐ion batteries (LIBs) with noncombustible solid‐state electrolytes (SSEs), we have the potential to fundamentally enhance safety measures. Concurrently, SSE would be capable of fitting high specific capacity (3860 mAh g −1 ) metal Li and is expected to break through the upper limit of mass‐energy density (350 Wh kg −1 ) of existing LIBs system. Nevertheless, the growth of Li dendrites on the negative side or the nucleation of Li inside SSEs may give rise to battery short circuits, which is the primary factor limiting the application of Li metal. Recognizing this, the focus of this review is to provide a perspective for experimentalists and theorists who closely monitor various surface/interface and microstructure phenomena to understand Li dendrites. The strategies to reveal the complicated deposition mechanism and to control the dendrite growth of metal Li in solid‐state batteries, as well as the advanced characterization methods of metal Li, provide suggestions for the practical research of solid‐state Li metal batteries.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.103
Threshold uncertainty score0.738

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.236
Teacher spread0.224 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations44
Published2024
Admission routes2
Has abstractyes

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