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Record W4391431264 · doi:10.1016/j.cej.2024.149142

Engineered biochar supported bismuth tungstate: Unveiling the influence of precursor concentrations and biochar dosage for the solar photocatalysis of 1,3-diphenylguanidine in secondary municipal effluent

2024· article· en· W4391431264 on OpenAlexafffund
Julide Kahkeci, Bouthaina Aoudi, Isaac Sánchez-Montes, Mohamed Gamal El‐Din

Bibliographic record

VenueChemical Engineering Journal · 2024
Typearticle
Languageen
FieldEnergy
TopicAdvanced Photocatalysis Techniques
Canadian institutionsUniversity of Alberta
FundersNatural Sciences and Engineering Research Council of CanadaMinistry of Economic Development and Trade, Government of AlbertaCanada Foundation for Innovation
KeywordsBiocharPhotocatalysisEffluentWastewaterTungstateDegradation (telecommunications)BismuthChemical engineeringMaterials scienceChemistryPulp and paper industryEnvironmental engineeringPyrolysisCatalysisInorganic chemistryEnvironmental scienceMetallurgyOrganic chemistry

Abstract

fetched live from OpenAlex

In this work, engineered hierarchal structures of biochar-supported bismuth tungstate are synthesized for wastewater treatment applications. The integration of biochar supports resulted in an increase in the surface area, reduction in crystallite size, and exposure of the active facets of Bi 2 WO 6 . Controlled Bi 2 WO 6 morphologies were obtained by varying the precursor concentrations, causing a remarkable transition from mixed microspheres to flower-like structures and, ultimately, to nanosheets. The optimal composite demonstrated its efficiency in a spiked wastewater secondary effluent, achieving 97.74 % degradation of 1,3-diphenylguanidine (DPG) under 8 h of simulated solar light irradiation. The treatment also reduced the toxicity and COD of the spiked secondary effluent matrix. The primary reactive oxygen species detected were O 2 •– and h + . Additionally, the photocatalytic degradation mechanism and possible degradation by-products of DPG were identified. These results highlight the significant influence of the biochar supports and synthesis parameters on the activity of biochar-supported photocatalysts, paving the way for the design of superior photocatalyst materials for wastewater treatment applications.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.040
Threshold uncertainty score0.646

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.245
Teacher spread0.237 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations30
Published2024
Admission routes2
Has abstractyes

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