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Record W4391436061 · doi:10.1016/j.fuel.2024.130994

Improving process sustainability in bio-oil transforming for biofuels and platform chemicals production: Valorization of the carbon residue

2024· article· en· W4391436061 on OpenAlexaff
Beatríz Valle, Roberto Palos, Iratxe Crespo, M. Mirari Antxustegi, Pedram Fatehi, María González Alriols

Bibliographic record

VenueFuel · 2024
Typearticle
Languageen
FieldEngineering
TopicBiodiesel Production and Applications
Canadian institutionsLakehead University
FundersH2020 Marie Skłodowska-Curie ActionsDiputación Foral de GipuzkoaMinisterio de Ciencia e InnovaciónEuropean Regional Development FundHorizon 2020 Framework ProgrammeEusko JaurlaritzaEuropean CommissionEuskal Herriko UnibertsitateaAgencia Estatal de InvestigaciónMinisterio de Ciencia, Innovación y Universidades
KeywordsBiofuelSustainabilityResidue (chemistry)Production (economics)Environmental sciencePulp and paper industryBiochemical engineeringSustainable productionOil productionBioenergyChemistryProcess (computing)Waste managementBusinessOrganic chemistryEconomicsComputer scienceEngineeringPetroleum engineeringEcology

Abstract

fetched live from OpenAlex

This work introduces a zero-waste approach to process biomass-derived raw bio-oil by addressing the valorization of the carbon residue that inevitably deposits, reducing the bio-oil conversion efficiency and leading to reactor-clogging issues. The study explores the feasibility of producing value-added porous material for removing pollutants from industrial wastewaters. An activated carbon with a specific surface area of 1070 m2 g−1 and a micropore volume of 0.41 mL g−1 was successfully produced through a simple thermochemical method involving pyrolysis, alkaline treatment, and carbonization. The impact that the activation method has on the nature, structure, and adsorption capacity of the material was assessed using methylene blue (MB) and hexavalent chromium (Cr-VI) as probe molecules. The activated carbon exhibited remarkable adsorption efficiency, achieving a removal ratio of 98 % for MB and 47 % for Cr-VI. Recyclability tests demonstrated a slight loss of adsorption capacity over multiple cycles. Kinetic studies, employing Surface Reaction Models and Mass Transfer Modeling, provide insights into adsorption rate-limiting steps. Chemisorption was identified as the most limiting stage, with physisorption and liquid film diffusion playing roles, particularly at short solid–liquid contact times. For longer contact times, intraparticle pore diffusion becomes the rate-controlling step due to the highly microporous nature of the activated carbon.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.285
Threshold uncertainty score0.231

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.236
Teacher spread0.226 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations5
Published2024
Admission routes1
Has abstractyes

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