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Record W4391493357 · doi:10.5194/amt-17-73-2024

New insights from the Jülich Ozone Sonde Intercomparison Experiment: calibration functions traceable to one ozone reference instrument

2024· article· en· W4391493357 on OpenAlexaff
H. G. J. Smit, Deniz Poyraz, Roeland Van Malderen, Anne M. Thompson, D. W. Tarasick, Ryan M. Stauffer, B. J. Johnson, Debra E. Kollonige

Bibliographic record

VenueAtmospheric measurement techniques · 2024
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicAtmospheric Ozone and Climate
Canadian institutionsEnvironment and Climate Change Canada
FundersBelgian Federal Science Policy Office
KeywordsOzoneCalibrationEnvironmental scienceConcentration cellCTDMeteorologyRemote sensingChemistryPhysicsMathematicsStatisticsGeographyElectrodeGeology

Abstract

fetched live from OpenAlex

Abstract. Although in principle ECC (electrochemical concentration cell) ozonesondes are absolute measuring devices, in practice they have several “artefacts” which change over the course of a flight. Most of the artefacts have been corrected in the recommendations of the Assessment of Standard Operating Procedures for Ozone Sondes (ASOPOS) report (Smit et al., 2021), giving an overall uncertainty of 5 %–10 % throughout the profile. However, the conversion of the measured cell current into the sampled ozone concentration still needs to be quantified better, using time-varying background current and more appropriate pump efficiencies. We describe an updated methodology for ECC sonde data processing that is based on the Jülich Ozone Sonde Intercomparison Experiment (JOSIE) 2009/2010 and JOSIE Southern Hemisphere Additional Ozonesondes (JOSIE-SHADOZ) 2017 test chamber data. The methodology resolves the slow and fast time responses of the ECC ozonesonde and in addition applies calibration functions to make the sonde data traceable to the JOSIE ozone reference UV photometer (OPM). The stoichiometry (O3/I2) factors and their uncertainties along with fast and slow reaction pathways for the different sensing solution types used in the global ozonesonde network are determined. Experimental evidence is given for treating the background current of the ECC sensor as the superposition of a constant ozone-independent component (IB0, measured before ozone exposure in the sonde preparation protocol) and a slow time-variant ozone-dependent current determined from the initial measured ozone current using a first-order numerical convolution. The fast sensor current is refined using the time response determined in sonde preparation with a first-order deconvolution scheme. Practical procedures for initializing the numerical deconvolution and convolution schemes to determine the slow and fast ECC currents are given. Calibration functions for specific ozonesondes and sensing solution type combinations were determined by comparing JOSIE 2009/2010 and JOSIE-SHADOZ 2017 profiles with the JOSIE OPM. With fast and slow currents resolved and the new calibration functions, a full uncertainty budget is obtained. The time response correction methodology makes every ozonesonde record traceable to one standard, i.e. the OPM of JOSIE, enabling the goal of a 5 % relative uncertainty to be met throughout the global ozone network.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.810
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0050.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.056
GPT teacher head0.246
Teacher spread0.190 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designNot applicable
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations22
Published2024
Admission routes1
Has abstractyes

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